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Optical Wave Mixing of Interacting Charge-Transfer Excitons in Organic Crystalline Films

机译:有机结晶膜中相互作用电荷转移激子的光波混合

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The nonlinear optical response of interacting charge-transfer excitons (CTEs) is investigated theoretically by means of pseudospin operators for the model Hamiltonian. The absorption and dispersion response of interacting CTEs associated with a weak probe field in the presence of a strong pump field is calculated in terms of the linear response theory. The numerical results are different from those of a driven two-level system with a weak probe and give a first example of gain without population inversion in a system of interacting CTEs.
机译:理论上通过用于模型Hamiltonian的伪旋转型操作员来研究相互作用电荷转移激子(CTE)的非线性光学响应。在线性响应理论方面计算与强泵场存在中的弱探针场相关联的相互作用CTE的吸收和分散响应。数值结果与具有弱探针的驱动的双级系统的数值不同,并在交互CTE的系统中提供没有群体反演的群体反演的第一示例。

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