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Physics of the metal-carbon nanotube interfaces: charge transfers, fermi-level 'pinning' and application to the scanning tunneling spectroscopy

机译:金属 - 碳纳米管界面的物理学:电荷转移,FERMI级“钉扎”和应用于扫描隧道光谱

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After its discovery in 1991, carbon nanotube has rapidly emerged as the most promising candidate for molecular electronics due to its quasi-one dimensional structure and the unique characterization of its electronic structure in terms of two simple geometric indices. Besides its huge technological potential, carbon nanotube also serves as the artificial laboratory in which one-dimensional transport can be investigated, similar to the semiconductor quantum wire. However, unlike its semiconductor cousin where transport is mostly ballistic, the study of transport in carbon nanotube has been distressed by the difficulty of making low resistance contact to the measuring electrodes. The high resistances reported in various two- and three-terminal measurements have led Tersoff (and also independently by one of the authors) to suggest that wavevector conservation at the metal-carbon nanotube contact may play an important role in explaining the high contact resistance. The complexity and importance of the metal-carbon nanotube interface makes it an immediate challenge to both theorists and experimentalists.
机译:在1991年发现之后,由于其准一维结构,碳纳米管迅速被作为分子电子的最有希望的候选者,并且在两个简单的几何指数方面是其电子结构的独特表征。除了其巨大的技术局部,碳纳米管还用作人工实验室,其中可以研究一维传输,类似于半导体量子线。然而,与其半导体表姐不同,其中运输大多是弹道,碳纳米管的运输研究通过使低电阻接触对测量电极而困扰。在各种两端和三端测量中报告的高电阻使得陶长约(并且也由其中一个作者独立)建议金属 - 碳纳米管接触处的波动保护可以在解释高接触电阻方面发挥重要作用。金属 - 碳纳米管界面的复杂性和重要性使其对理论家和实验主义者来说是一种立即挑战。

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