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NONSEQUENTIAL DOUBLE IONIZATION: A MINIMAL -CORRELATION APPROACH

机译:非顺序的双电离:最小的 - 胶合方法

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Nonsequential multiple ionization, where two or more electrons are ripped off the atom by the laser field in one coherent process, has attracted much interest for over a decade. Representative references include for experimental data and [7-16] for theoretical work; the not-too-recent work is covered in the review articles. Unlike above-threshold ionization (ATI) or higli-harmonic generation (HHG), this process cannot proceed in the absence of electron-electron correlation. Moreover, this correlation affords a sizeable premiu n for collaboration between the two electrons: for optimal laser intensities, the ratio of nonsequential over sequential double ionization, which materializes in the famous "knee", can be as high as six orders of magnitude. Until about a year ago, experimental data were restricted to the total yields. Recently, however, application of the COLTRIMS (cold-target recoil-ion-momentum spectroscopy) technique has allowed for the determination of the (three-dimensional) momenta of the ion and the electrons so that now the completely differential ionization rate has become accessible. Early on, rescattering was identified as a promising candidate for the physical mechanism of nonsequential double ionization (NSDI), the same mechanism that is known to be responsible for ATI and HHG. However, serious quantitative problems with this scenario precluded its acceptance until recently. This problem has now been revisited and appears to have been reso ved. More and more, rescattering is emerging as the dominant mechanism, but depending on the atomic species and the laser intensity, others may be required in addition. Thus far, there are only few theoretical results for the momentum distributions in NSDI and even fewer explicit calculations. The intense-field many-particle 5-matrix theory which has successfully reproduced many data for the total yields has been extended to calculations of the differential rates. A calcu-lationally simpler version of essentially the same model yields similar results in those parameter regimes where it is applicable. There is also a simulation on the basis of the time-dependent Schroedinger equation in one dimension for each electron. Much can be learned already from purely classical kinematical considerations along the lines of the so-called simple-man model of intense -laser atom processes. In this paper, we present a simple fully quantum-mechanical model hat is able to predict the momentum distributions for any given scenario, such as sequential ionization, nonsequential ionization via rescattering, or nonsequential ioniza-tion via rescattering into an excited state followed by tunneling. The absolute yield for a given scenario cannot be predicted, but its intensity dependence can. Most importantly, different scenarios generate very different momentum distributions. Comparison of the calculated with the measured momentum distributions then can support or discredit the respective scenario.
机译:非顺序多电离,其中两个或多个电子通过激光场在一个相干过程中从原子上撕下原子,在十年上吸引了很多兴趣。代表参考包括实验数据和[7-16]用于理论上;审查文章中涵盖了不太最近的工作。与上阈值电离(ATI)或HIGLI-谐波产生(HHG)不同,该过程不能在没有电子相关的情况下进行。此外,这种相关性为两个电子之间的合作提供了相同的预测,用于最佳激光强度,在着名的“膝关节”中实现的连续双电离的非顺序比的比率可以高达六个数量级。直到一年前,实验数据仅限于总产量。然而,近来,允许Coltrims(冷 - 目标反冲 - 离子动量光谱)技术的应用,用于确定离子的(三维)电影和电子,以便现在完全差分电离率已变得可访问。早期,鉴定了resmattering作为非顺强性双电离(NSDI)的物理机制的有希望的候选者,该具有相同的机制是由ATI和HHG负责的。然而,这种情况的严重量化问题排除了其接受直到最近。现在已经重新审视了这个问题,似乎是ved。越来越多地,振选被涌现为主要机制,但取决于原子物种和激光强度,另外可能还需要。到目前为止,NSDI中的动量分布甚至甚至明确的计算甚至都有很少的理论结果。已经成功复制了总收益率的许多数据的激烈场多粒子5矩阵理论已经扩展到差分速率的计算。基本上相同的模型的Calcu合理的版本在适用的参数制度中产生类似的结果。在每个电子的一个尺寸中,还存在基于时间依赖的Schroedinger方程的模拟。已经可以从纯粹的经典运动考虑到沿着强烈的激烈的激烈原子进程的所谓简单的模型的线条学习了很多。在本文中,我们介绍了一个简单的全量子机械模型帽,能够通过校正隧道,从而预测任何给定场景的动量分布,例如通过调节,或非顺强的离子化,或者是非顺强的离子化,或者通过校正隧道。不能预测给定方案的绝对收益率,但其强度依赖性可以。最重要的是,不同的场景产生非常不同的动量分布。用测量的动量分布计算的比较然后可以支持或诋毁相应的情景。

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