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Comparison of stimulated Raman scattering of picosecond pulses in tungsten crystals

机译:钨晶体中皮秒脉冲受激拉曼散射的比较

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Abstract: Stimulated Raman scattering of picosecond pulses was investigated in KGd(WO$-4$/)$-2$/, and BaWO$-4$/ tungstate crystals. BaWO$-4$/ crystal was previously found to be a new very efficient material for pumping with nanosecond pulses. In our experiment, we used the second harmonic output of a mode-locked Nd:YAG laser system, which generated single pulses of 28 ps duration. The length of the crystal was 40 mm for KGW, 23 mm for KYW and 29 mm for BaWO$-4$/. The SRS threshold, conversion efficiency, and time dependence of the first Stokes with picosecond resolution were measured. Picosecond Raman gains at a 532 nm wavelength were found to be correspondingly 11.5, 18.7, and 14.4 cm/GW for KGW, KYW, and BaWO$-4$/. The Raman shifting up to the third Stokes component was detected, and the first Stokes conversion efficiency reached 30 percent in BaWO$-4$/ and 18 percent in KGd(WO$-4$/)$-2$/. Measurements of a temporal pulse length have shown that the first Stokes pulse was twice shorter than the pump pulse. The new BaWO$-4$/ crystal occurs to be an efficient solid state Raman material for a wide variety of pump pulse durations. !19
机译:摘要:研究了钨酸盐晶体KGd(WO $ -4 $ /)$-2 $ /和BaWO $ -4 $ /皮秒脉冲的受激拉曼散射。以前发现BaWO $ -4 $ /晶体是一种新型的非常有效的材料,用于泵浦纳秒脉冲。在我们的实验中,我们使用了锁模Nd:YAG激光系统的二次谐波输出,该系统生成了持续时间为28 ps的单个脉冲。对于KGW,晶体的长度为40毫米,对于KYW,晶体的长度为23毫米,对于BaWO $ -4 $ /,晶体的长度为29毫米。测量了具有皮秒分辨率的第一个Stoke的SRS阈值,转换效率和时间依赖性。对于KGW,KYW和BaWO $ -4 $ /,发现在532 nm波长处的皮秒拉曼增益分别为11.5、18.7和14.4 cm / GW。检测到拉曼移至第三斯托克斯分量,并且第一斯托克斯转换效率在BaWO $ -4 $ /中达到30%,在KGd(WO $ -4 $ /)$-2 $ /中达到18%。时间脉冲长度的测量表明,第一个斯托克斯脉冲比泵浦脉冲短两倍。新的BaWO $ -4 $ /晶体是一种有效的固态拉曼材料,适用于各种泵浦脉冲持续时间。 !19

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