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Terahertz emission from gold nanorods irradiated by ultrashort laser pulses of different wavelengths

机译:不同波长的超短激光脉冲照射的金纳米棒的太赫兹发射

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摘要

Electron photoemission and ponderomotive acceleration by surface enhanced optical fields is considered as a plausible mechanism of terahertz radiation from metallic nanostructures under ultrafast laser excitation. To verify this mechanism, we studied experimentally terahertz emission from an array of gold nanorods illuminated by intense (~10–100 GW/cm2) femtosecond pulses of different central wavelengths (600, 720, 800, and 1500 nm). We found for the first time that the order of the dependence of the terahertz fluence on the laser intensity is, unexpectedly, almost the same (~4.5–4.8) for 720, 800, and 1500 nm and somewhat higher (~6.6) for 600 nm. The results are explained by tunneling currents driven by plasmonically enhanced laser field. In particular, the pump-intensity dependence of the terahertz fluence is more consistent with terahertz emission from the sub-cycle bursts of the tunneling current rather than with the ponderomotive mechanism.
机译:通过表面增强光场进行的电子光发射和质子加速被认为是超快激光激发下金属纳米结构的太赫兹辐射的合理机制。为了验证这种机制,我们通过实验研究了由金纳米棒阵列中的太赫兹发射,这些金纳米棒由不同中心波长(600、720、800和1500)。我们首次发现,太赫兹注量对激光强度的依赖性出乎意料的是,对于720、800和1500 nm,它几乎相同(〜4.5-4.8),而对于600 600nm则更高(〜6.6)纳米结果由等离子体增强激光场驱动的隧穿电流解释。特别地,太赫兹注量的泵浦强度依赖性与隧道电流的子周期突发中的太赫兹发射更一致,而不是与致动力机制更一致。

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