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Interplay of relativistic and nonrelativistic transport in atomically precise segmented graphene nanoribbons

机译:原子精确分割的石墨烯纳米带中相对论和非相对论传输的相互作用

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摘要

Graphene's isolation launched explorations of fundamental relativistic physics originating from the planar honeycomb lattice arrangement of the carbon atoms, and of potential technological applications in nanoscale electronics. Bottom-up fabricated atomically-precise segmented graphene nanoribbons, SGNRs, open avenues for studies of electrical transport, coherence, and interference effects in metallic, semiconducting, and mixed GNRs, with different edge terminations. Conceptual and practical understanding of electric transport through SGNRs is gained through nonequilibrium Green's function (NEGF) conductance calculations and a Dirac continuum model that absorbs the valence-to-conductance energy gaps as position-dependent masses, including topological-in-origin mass-barriers at the contacts between segments. The continuum model reproduces the NEGF results, including optical Dirac Fabry-Prot (FP) equidistant oscillations for massless relativistic carriers in metallic armchair SGNRs, and an unequally-spaced FP pattern for mixed armchair-zigzag SGNRs where carriers transit from a relativistic (armchair) to a nonrelativistic (zigzag) regime. This provides a unifying framework for analysis of coherent transport phenomena and interpretation of forthcoming experiments in SGNRs.
机译:石墨烯的隔离引发了对相对论物理学的探索,这些物理学起源于碳原子的平面蜂窝晶格排列,还探索了纳米级电子学中的潜在技术应用。自下而上的原子精确分段石墨烯纳米带,SGNRs,是研究金属,半导体和混合GNRs中具有不同边缘端接的电传输,相干性和干扰效应的开放途径。通过非平衡格林函数(NEGF)电导计算和Dirac连续模型,可以吸收价电导能隙作为与位置相关的质量,包括起源于拓扑的质量屏障,从而获得了通过SGNRs进行电传输的概念和实践理解。在段之间的接触处。连续体模型再现了NEGF结果,包括金属扶手椅SGNR中无质量相对论载体的光学Dirac Fabry-Prot(FP)等距振荡,以及混合扶手椅-曲折SGNR的不等距FP模式,其中载体从相对论(扶手椅)过渡转向非相对论(之字形)政体。这为分析相干传输现象和解释SGNR中即将进行的实验提供了一个统一的框架。

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