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The Chemistry and Promising Applications of Graphene and Porous Graphene Materials

机译：石墨烯和多孔石墨烯材料的化学和有前途的应用

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摘要

Graphene and graphene oxide (GO), as wonder materials, have penetrated nearly every field of research. One of their most attractive features is the functionality and assembly of graphene or GO, in which they can be considered to be chemically functionalized building blocks for creating unconventional porous graphene materials (PGMs) that not only combine the merits of both porous materials and graphene, but also have major advantages over other porous carbons for specific applications. The chemistry and approaches for functionalizing graphene and GO are first introduced, and typical procedures for pore creation (e.g., in-plane pores, 2D laminar pores, and 3D interconnected pore assemblies), self-assembly, and tailoring mechanisms for PGMs to highlight the significance of precise control over the pore morphology and pore size are summarized. Because of their unique pore structures, with different morphologies and intriguing properties, PGMs serve as key components in a variety of applications such as energy storage, electrocatalysis, and molecular separation. Finally, the challenges relating to PGMs from the understanding of chemical self-assembly to specific applications are discussed, and promising solutions on how to tackle them are presented. This provides an insightful outlook for the future development of the chemistry and applications of PGMs.
机译：石墨烯和石墨烯氧化物（GO），作为神奇的材料，几乎渗透了几乎每个研究领域。其中一个最具吸引力的特点是石墨烯或Go的功能和组装，其中它们可以被认为是用于产生非传统多孔石墨烯材料（PGMS）的化学官能化的构建块，其不仅结合了多孔材料和石墨烯的优点，而且还具有对特定应用的其他多孔碳的主要优点。首先介绍了官能化石墨烯和官能化的化学和方法，以及用于PGM的自动组装和剪裁机制的孔创建（例如，面内孔，2D层孔和3D互连的孔组装的典型方法。总结了精确控制对孔形态和孔径的重要性。由于其独特的孔隙结构，具有不同的形态和有趣性质，PGMS作为各种应用中的关键部件，例如储能，电常见和分子分离。最后，讨论了与对特定应用的理解有关PGM的挑战，并提出了有关如何解决它们的承诺解决方案。这为未来的化学和PGM应用的发展提供了洞察力。

著录项

  • 来源
    《Advanced Functional Materials》 |2020年第41期|1909035.1-1909035.39|共39页
  • 作者

    Huang Haibo; Shi Haodong; Das Pratteek; Qin Jieqiong; Li Yaguang; Wang Xiao; Su Feng; Wen Pengchao; Li Suyuan; Lu Pengfei; Liu Fangyan; Li Yuejiao; Zhang Ying; Wang Yi; Wu Zhong-Shuai; Cheng Hui-Ming;

  • 作者单位

    Chinese Acad Sci Dalian Inst Chem Phys Dalian Natl Lab Clean Energy 457 Zhongshan Rd Dalian 116023 Peoples R China;

    Chinese Acad Sci Dalian Inst Chem Phys Dalian Natl Lab Clean Energy 457 Zhongshan Rd Dalian 116023 Peoples R China|Univ Chinese Acad Sci Beijing 100049 Peoples R China;

    Chinese Acad Sci Dalian Inst Chem Phys Dalian Natl Lab Clean Energy 457 Zhongshan Rd Dalian 116023 Peoples R China|Univ Chinese Acad Sci Beijing 100049 Peoples R China;

    Chinese Acad Sci Dalian Inst Chem Phys Dalian Natl Lab Clean Energy 457 Zhongshan Rd Dalian 116023 Peoples R China|Univ Chinese Acad Sci Beijing 100049 Peoples R China;

    Chinese Acad Sci Dalian Inst Chem Phys Dalian Natl Lab Clean Energy 457 Zhongshan Rd Dalian 116023 Peoples R China;

    Chinese Acad Sci Dalian Inst Chem Phys Dalian Natl Lab Clean Energy 457 Zhongshan Rd Dalian 116023 Peoples R China|Univ Chinese Acad Sci Beijing 100049 Peoples R China;

    Chinese Acad Sci Dalian Inst Chem Phys Dalian Natl Lab Clean Energy 457 Zhongshan Rd Dalian 116023 Peoples R China|Univ Chinese Acad Sci Beijing 100049 Peoples R China;

    Chinese Acad Sci Dalian Inst Chem Phys Dalian Natl Lab Clean Energy 457 Zhongshan Rd Dalian 116023 Peoples R China;

    Chinese Acad Sci Dalian Inst Chem Phys Dalian Natl Lab Clean Energy 457 Zhongshan Rd Dalian 116023 Peoples R China;

    Chinese Acad Sci Dalian Inst Chem Phys Dalian Natl Lab Clean Energy 457 Zhongshan Rd Dalian 116023 Peoples R China;

    Chinese Acad Sci Dalian Inst Chem Phys Dalian Natl Lab Clean Energy 457 Zhongshan Rd Dalian 116023 Peoples R China;

    Chinese Acad Sci Dalian Inst Chem Phys Dalian Natl Lab Clean Energy 457 Zhongshan Rd Dalian 116023 Peoples R China;

    Chinese Acad Sci Dalian Inst Chem Phys Dalian Natl Lab Clean Energy 457 Zhongshan Rd Dalian 116023 Peoples R China|Univ Chinese Acad Sci Beijing 100049 Peoples R China;

    Chinese Acad Sci Dalian Inst Chem Phys Dalian Natl Lab Clean Energy 457 Zhongshan Rd Dalian 116023 Peoples R China|Univ Chinese Acad Sci Beijing 100049 Peoples R China;

    Chinese Acad Sci Dalian Inst Chem Phys Dalian Natl Lab Clean Energy 457 Zhongshan Rd Dalian 116023 Peoples R China;

    Chinese Acad Sci Inst Met Res Shenyang Natl Lab Mat Sci Shenyang 110016 Peoples R China|Tsinghua Univ Tsinghua Berkeley Shenzhen Inst Shenzhen 518055 Peoples R China|Univ Surrey Adv Technol Inst Guildford GU2 7XH Surrey England;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    applications; chemistry; graphene; graphene oxide; porous materials;

    机译：应用;化学;石墨烯;石墨烯;多孔材料;

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