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Solution-Processed Highly Efficient Alternating Current-Driven Field-Induced Polymer Electroluminescent Devices Employing High-k Relaxor Ferroelectric Polymer Dielectric

机译:采用高k弛豫铁电聚合物介电材料的固溶处理高效交流电驱动场致聚合物电致发光器件

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摘要

Organic thin-film electroluminescent (EL) devices, such as organic light-emitting diodes (OLEDs), typically operate using constant voltage or direct current (DC) power sources. Such approaches require power converters (introducing power losses) and make devices sensitive to dimensional variations that lead to run away currents at imperfections. Devices driven by time-dependent voltages or alternating current (AC) may offer an alternative to standard OLED technologies. However, very little is known about how this might translate into overall performance of such devices. Here, a solution-processed route to creating highly efficient AC field-induced polymer EL (FIPEL) devices is demonstrated. Such solution-processed FIPEL devices show maximum luminance, current efficiency, and power efficiency of 3000 cd m~(-2),15.8 cd A~(-1), and 3.1 lm W~(-1) for blue emission, 13 800 cd m~(-2), 76.4 cd A~(-1), and 17.1 lm W~(-1) for green emission, and 1600 cd m~(-2),8.8 cd A~(-1), and 1.8 l W~(-1) for orange-red emission. The high luminance and efficiency, and solution process pave the way to industrial roll-to-roll manufacturing of solid state lighting and display.
机译:有机薄膜电致发光(EL)器件(例如有机发光二极管(OLED))通常使用恒定电压或直流(DC)电源运行。这种方法需要功率转换器(引入功率损耗),并使设备对尺寸变化敏感,从而导致缺陷处的电流失控。由随时间变化的电压或交流电(AC)驱动的设备可以提供标准OLED技术的替代产品。但是,对于如何将其转化为此类设备的整体性能知之甚少。在此,说明了通过溶液处理的方法来创建高效的交流场感应聚合物EL(FIPEL)器件。此类溶液处理的FIPEL器件显示出最大亮度,电流效率和功率效率,分别为3000 cd m〜(-2),15.8 cd A〜(-1)和3.1 lm W〜(-1),发射蓝色光为13800 cd m〜(-2),76.4 cd A〜(-1)和17.1 lm W〜(-1)用于绿色发射,以及1600 cd m〜(-2),8.8 cd A〜(-1)和1.8 l W〜(-1)用于橙红色发射。高亮度和高效率以及解决方案工艺为固态照明和显示器的工业卷对卷制造铺平了道路。

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  • 来源
    《Advanced Functional Materials》 |2014年第11期|1501-1508|共8页
  • 作者单位

    Center for Nanotechnology and Molecular Materials Department of Physics Wake Forest University Winston-Salem, NC 27105, USA;

    Center for Nanotechnology and Molecular Materials Department of Physics Wake Forest University Winston-Salem, NC 27105, USA;

    State Key Laboratory of Polymer Physics and Chemistry Changchun Institute of Applied Chemistry Chinese Academy of Sciences Changchun 130022, P. R. China;

    Center for Nanotechnology and Molecular Materials Department of Physics Wake Forest University Winston-Salem, NC 27105, USA;

    State Key Laboratory of Polymer Physics and Chemistry Changchun Institute of Applied Chemistry Chinese Academy of Sciences Changchun 130022, P. R. China;

    State Key Laboratory of Polymer Physics and Chemistry Changchun Institute of Applied Chemistry Chinese Academy of Sciences Changchun 130022, P. R. China;

    Center for Nanotechnology and Molecular Materials Department of Physics Wake Forest University Winston-Salem, NC 27105, USA;

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