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Ultrahigh Responsivity of Ternary Sb-Bi-Se Nanowire Photodetectors

机译:三元Sb-Bi-Se纳米线光电探测器的超高响应度

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摘要

High-quality single-crystalline ternary (Sb_(1-x)Bi_x)_2Se_3 nanowires (NWs) (x = 0-0.88) are synthesized by chemical vapor deposition. Nanowires with x from 0 to 0.75 are indexed as an orthorhombic structure. With increasing Bi incorporation ratio, (Sb_(1-x)Bi_x)_2Se_3 NWs exhibit remarkable photoresponsivities, which originate from growing surface Se vacancies and augmented oxygen chemisorptions. Notably, spectra responsivity and external quantum efficiency of an (Sb_(0.44)Bi_(0.56))_2Se_3 NW photodetector reach as high as ≈8261.4 A/W and ≈1.6 × 10~6 %, respectively. Those excellent performances unambiguously demonstrate that Sb-Bi-Se NWs are promising for the utilizations of high-sensitivity and high-speed photodetectors and photoelectronic switches.
机译:通过化学气相沉积法合成了高质量的单晶三元(Sb_(1-x)Bi_x)_2Se_3纳米线(NWs)(x = 0-0.88)。 x从0到0.75的纳米线被索引为正交结构。随着Bi掺入比例的增加,(Sb_(1-x)Bi_x)_2Se_3 NWs表现出显着的光响应性,其起因于表面硒空位的增加和氧化学吸附的增加。值得注意的是,(Sb_(0.44)Bi_(0.56))_ 2Se_3 NW光电探测器的光谱响应度和外部量子效率分别高达≈8261.4A / W和≈1.6×10〜6%。这些出色的性能清楚地表明,Sb-Bi-Se纳米线在使用高灵敏度,高速光电探测器和光电开关方面很有前途。

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  • 来源
    《Advanced Functional Materials》 |2014年第23期|3581-3586|共6页
  • 作者单位

    Suzhou Institute of Nano-Tech and Nano-Bionics Chinese Academy of Sciences 398 Ruoshui Road, Suzhou Industrial Park Jiangsu 215123, China,University of Chinese Academy of Sciences 19A Yuquan Road, Beijing 100049, China;

    Suzhou Institute of Nano-Tech and Nano-Bionics Chinese Academy of Sciences 398 Ruoshui Road, Suzhou Industrial Park Jiangsu 215123, China,University of Chinese Academy of Sciences 19A Yuquan Road, Beijing 100049, China;

    Suzhou Institute of Nano-Tech and Nano-Bionics Chinese Academy of Sciences 398 Ruoshui Road, Suzhou Industrial Park Jiangsu 215123, China,University of Chinese Academy of Sciences 19A Yuquan Road, Beijing 100049, China;

    Suzhou Institute of Nano-Tech and Nano-Bionics Chinese Academy of Sciences 398 Ruoshui Road, Suzhou Industrial Park Jiangsu 215123, China;

    Suzhou Institute of Nano-Tech and Nano-Bionics Chinese Academy of Sciences 398 Ruoshui Road, Suzhou Industrial Park Jiangsu 215123, China;

    Suzhou Institute of Nano-Tech and Nano-Bionics Chinese Academy of Sciences 398 Ruoshui Road, Suzhou Industrial Park Jiangsu 215123, China;

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