Heterogeneous graphene oxide as recyclable catalyst for azomethine ylide mediated 1,3 dipolar cycloaddition reaction in aqueous medium

Marri Sameer Reddy; Nandigama Satish Kumar; L. Raju Chowhan

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Heterogeneous graphene oxide as recyclable catalyst for azomethine ylide mediated 1,3 dipolar cycloaddition reaction in aqueous medium

机译：非均相氧化石墨烯作为可循环催化剂在水性介质中偶氮甲内酯介导的1,3偶极环加成反应

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Graphene oxide (GO) catalysed multi component reaction of azomethine ylide driven 1,3 dipolar cycloaddition reaction in aqueous ethanolic solution is reported for the first time. This strategy has been applied for the synthesis of poly heterocyclic spiro-indenoquinoxaline pyrrolizidines and spiro-oxindoles pyrrolizidines with good to excellent yield along with excellent regio and diastereoselectivity. An ultra-low catalyst loading of 0.50?wt% was found to be efficient to catalyse the reaction.

机译：首次报道了在乙醇水溶液中氧化石墨烯（GO）催化的甲亚胺叶立德驱动的1,3偶极环加成反应的多组分反应。该策略已被用于合成具有良好或优异的收率以及优异的区域和非对映选择性的多杂环螺-茚并喹喔啉吡咯并核苷和螺-羟吲哚吡咯并核苷的合成。发现0.50wt％的超低催化剂负载量对催化反应是有效的。

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《RSC Advances》 |2018年第62期|共7页
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Marri Sameer Reddy; Nandigama Satish Kumar; L. Raju Chowhan;
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1. Heterogeneous graphene oxide as recyclable catalyst for azomethine ylide mediated 1,3 dipolar cycloaddition reaction in aqueous medium [J] . Reddy Marri Sameer, Kumar Nandigama Satish, Chowhan L. Raju RSC Advances . 2018,第62期

机译：非均相石墨烯氧化物作为可回收催化剂用于氮杂甲酸钠ylide介导的含水介质中的1,3偶极环加入反应
2. Heterogeneous graphene oxide as recyclable catalyst for azomethine ylide mediated 1,3 dipolar cycloaddition reaction in aqueous medium [J] . Marri Sameer Reddy, Nandigama Satish Kumar, L. Raju Chowhan RSC Advances . 2018,第62期

机译：非均相氧化石墨烯作为可循环催化剂在水性介质中偶氮甲内酯介导的1,3偶极环加成反应
3. INFLUENCE OF AG(I) AND LI(I) CATALYSTS FOR 1,3-DIPOLAR CYCLOADDITION REACTIONS OF AZOMETHINE YLIDES - REVERSAL OF THE STEREOCHEMISTRY [J] . Nyerges M., Toth G., Herenyi B., Tetrahedron . 1995,第48期

机译：AG（I）和Li（I）催化剂对偶氮嘧啶盐1,3-二氯环化反应的影响-立体化学的逆转
4. REGIOSELECTIVITY IN 1,3-DIPOLAR CYCLOADDITION REACTIONS OF PYRIMIDINIUM-N-YLIDES TO ALKYNES(Abstracts) [C] . Florentina Georgescu, Emilian Georgescu, Constantin Roibu European Symposium on Organic Chemistry . 2007

机译：嘧啶-N-ylides至alkynes（摘要）的1,3-偶极环加成反应的区域选择性
5. 1,3-Dipolar cycloaddition of azomethine ylides to carbon(60) and carbon(70): Combinatorial synthesis of a small library of pyridazines using polymer-bound azodicarboxylate resin. [D] . Tan, Xuefei. 2002

机译：1,3-偶极亚甲基环向碳（60）和碳（70）的偶极环加成反应：使用聚合物结合的偶氮二羧酸酯树脂组合合成一个小的哒嗪类文库。
6. A Novel One-Pot Green Synthesis of Dispirooxindolo-pyrrolidines via13-Dipolar Cycloaddition Reactions of Azomethine Ylides [O] . Abdulrahman I. Almansour, Natarajan Arumugam, Raju Suresh Kumar, 2015

机译：通过偶氮甲Y叶立德的13-偶极环加成反应合成新颖的一锅绿色双螺并吡咯并吡咯烷类化合物
7. Heterogeneous graphene oxide as recyclable catalyst for azomethine ylide mediated 1,3 dipolar cycloaddition reaction in aqueous medium [O] . Marri Sameer Reddy, Nandigama Satish Kumar, L. Raju Chowhan 2018

机译：非均相石墨烯氧化物作为可回收催化剂用于氮杂甲酸钠ylide介导的含水介质中的1,3偶极环加入反应

Heterogeneous graphene oxide as recyclable catalyst for azomethine ylide mediated 1,3 dipolar cycloaddition reaction in aqueous medium

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