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Carbonaceous layer interfaced TiO2/RGO hybrids with enhanced visible-light photocatalytic performance

机译:碳质层接口TiO2 / RGO杂交物,具有增强的可见光光催化性能

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A facile solvothermal method combined with heat treatment was introduced to obtain enhanced photocatalytic activity of TiO _(2) @C/RGO (reduced graphene oxide) photocatalyst under visible light. By adjusting the annealing temperature, the physical and chemical status of the interfacial carbonaceous layer could be successfully tuned. The carbonaceous layer with optimal thickness and degree of order obtained at 360 °C forms a good bridge between the TiO _(2) particles and RGO sheet. The resulting TiO _(2) @C-360/RGO photocatalyst exhibited the best performance in the photodegradation of MO under visible light, benefiting from the ideal connection provided by the optimal carbonaceous layer and thus enhanced separation of activated electron–hole pairs at the interface. In addition, the photocatalytic activity was adjusted synchronously by controlling the thickness and degree of order of the carbonaceous layer in the TiO _(2) @C/RGO hybrids. This work indicates the importance of interface engineering to obtain TiO _(2) -based nanohybrids with high photocatalytic performance.
机译:引入与热处理结合热处理的容易溶剂热法以在可见光下获得TiO _(2)℃/ rgo(氧化物还原)光催化剂的增强的光催化活性。通过调节退火温度,可以成功调整界面碳质层的物理和化学状态。在360℃下获得的最佳厚度和最佳厚度的碳质层在TiO _(2)颗粒和RGO板之间形成良好的桥梁。得到的TiO _(2)/ @ C-360 / RGO光催化剂在可见光下的MO光降解中表现出最佳性能,受益于最佳碳质层提供的理想连接,从而增强了活化的电子孔对的分离界面。另外,通过控制TiO _(2)℃/ rgo杂种的碳质层的厚度和阶阶段同步地同步地调节光催化活性。这项工作表明界面工程的重要性,以具有高光催化性能的基于纳米次组获得TiO _(2)。

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