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Hormones and Pharmaceuticals in Groundwater Used As a Source of Drinking Water Across the United States

机译:全美用作饮用水源的地下水中的激素和药物

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摘要

This is the first large-scale, systematic assessment of hormone and pharmaceutical occurrence in groundwater used for drinking across the United States. Samples from 1091 sites in Principal Aquifers representing 60% of the volume pumped for drinking-water supply had final data for 21 hormones and 103 pharmaceuticals. At least one compound was detected at 5.9% of 844 sites representing the resource used for public supply across the entirety of 15 Principal Aquifers, and at 11.3% of 247 sites representing the resource used for domestic supply over subareas of nine Principal Aquifers. Of 34 compounds detected, one plastics component (bisphenol A), three pharmaceuticals (carbamazepine, sulfamethoxazole, and meprobamate), and the caffeine degradate 1,7-dimethylxanthine were detected in more than 0.5% of samples. Hydrocortisone had a concentration greater than a human-health benchmark at 1 site. Compounds with high solubility and low K-oc were most likely to be detected. Detections were most common in shallow wells with a component of recent recharge, particularly in crystalline-rock and mixed land-use settings. Results indicate vulnerability of groundwater used for drinking water in the U.S. to contamination by these compounds is generally limited, and exposure to these compounds at detected concentrations is unlikely to have adverse effects on human health.
机译:这是在美国范围内首次大规模,系统地评估用于饮用水的地下水中激素和药物的存在。来自主要含水层中1091个位置的样品占饮用水抽取量的60%,具有21种激素和103种药物的最终数据。在15个主要含水层的844个站点中,至少有一种化合物被检测为公共供应资源;在9个主要含水层的子区域中,检测到了247个站点中的11.3%,其代表了国内供应资源。在检测到的34种化合物中,在超过0.5%的样品中检测到一种塑料成分(双酚A),三种药物(卡马西平,磺胺甲恶唑和甲丙氨酯)和咖啡因降解的1,7-二甲基黄嘌呤。 1个地点的氢化可的松浓度高于人类健康基准。具有高溶解度和低K-oc的化合物最有可能被检测到。在带有最近补给成分的浅井中,检测最常见,尤其是在晶体岩和混合土地利用环境中。结果表明,在美国,用于饮用水的地下水对这些化合物污染的脆弱性通常受到限制,并且以检测到的浓度暴露于这些化合物不太可能对人体健康产生不利影响。

著录项

  • 来源
    《Environmental Science & Technology》 |2019年第6期|2950-2960|共11页
  • 作者单位

    US Geol Survey, 6700 Edith Blvd NE, Albuquerque, NM 87113 USA;

    US Geol Survey, 6000 J St,Placer Hall, Sacramento, CA 95819 USA;

    US Geol Survey, 10 Bearfoot Rd, Northborough, MA 01532 USA;

    US Geol Survey, Denver Fed Ctr, POB 25585, Denver, CO 80225 USA;

    US Geol Survey, Denver Fed Ctr, POB 25585, Denver, CO 80225 USA;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
  • 原文格式 PDF
  • 正文语种 eng
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