Methanol from CO_2 by Organo-Cocatalysis: CO_2 Capture and Hydrogenation in One Process Step

Christian Reller; Matthias Poege; Andreas Lissner; Florian O. R. L Mertens

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Methanol from CO_2 by Organo-Cocatalysis: CO_2 Capture and Hydrogenation in One Process Step

机译：有机共催化从CO_2中制取甲醇：一步法完成CO_2的捕获和氢化

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摘要

Carbon dioxide chemically bound to alcohol-amines was hydrogenated to methanol under retrieval of these industrially used CO_2 capturing reagents. The energetics of the process can be seen as a partial cancellation of the exothermic heat of reaction of the hydrogenation with the endothermic one of the CO_2 release from the capturing reagent. The process provides a means to significantly improve the energy efficiency of CO_2 to methanol conversions.

机译：在回收这些工业上使用的CO_2捕获试剂的过程中，将与醇胺化学键合的二氧化碳氢化为甲醇。该方法的能量学可以看作是氢化反应与从捕获剂中释放出的CO 2之一的吸热反应的放热反应的部分抵消。该方法提供了一种显着提高CO_2转化为甲醇的能效的方法。

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《Environmental Science & Technology》 |2014年第24期|14799-14804|共6页
作者
Christian Reller; Matthias Poege; Andreas Lissner; Florian O. R. L Mertens;
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作者单位

Institut fuer Physikalische Chemie, Technische Universitaet Bergakademie Freiberg, Leipziger Strasse 29, 09599 Freiberg, Germany;

Institut fuer Physikalische Chemie, Technische Universitaet Bergakademie Freiberg, Leipziger Strasse 29, 09599 Freiberg, Germany;

Institut fuer Physikalische Chemie, Technische Universitaet Bergakademie Freiberg, Leipziger Strasse 29, 09599 Freiberg, Germany;

Institut fuer Physikalische Chemie, Technische Universitaet Bergakademie Freiberg, Leipziger Strasse 29, 09599 Freiberg, Germany;

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收录信息美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
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专利

1. Integrative CO_2 Capture and Hydrogenation to Methanol with Reusable Catalyst and Amine: Toward a Carbon Neutral Methanol Economy [J] . Sayan Kar, Raktim Sen, Alain Goeppert, Journal of the American Chemical Society . 2018,第5期

机译：通过可重复使用的催化剂和胺将CO_2捕获和加氢制为甲醇：实现碳中和甲醇经济
2. Thermodynamic assessment of zero-emission power, hydrogen and methanol production using captured CO_2 from S-Graz oxy-fuel cycle and renewable hydrogen [J] . Nami Hossein, Ranjbar Faramarz, Yari Mortaza Energy Conversion & Management . 2018,第APRa期

机译：使用从S-Graz含氧燃料循环中捕获的CO_2和可再生氢，对零排放功率，氢和甲醇生产进行热力学评估
3. Ca_2Fe_2O_5: A promising oxygen carrier for CO/CH_4 conversion and almost- pure H_2 production with inherent CO_2 capture over a two-step chemical looping hydrogen generation process [J] . Sun Zhao, Chen Shiyi, Hu Jun, Applied Energy . 2018,第FEBa1期

机译：Ca_2Fe_2O_5：一种有前途的氧气载体，可用于CO / CH_4转化和几乎纯净的H_2生产，并通过两步化学循环制氢工艺捕获固有的CO_2
4. CAMERE Process for methanol synthesis from CO_2 hydrogenation [C] . International Conference on Carbon Dioxide Utilization . 2004

机译：COMERE用于甲醇合成的CO_2氢化
5. High temperature reactive separation process for combined carbon dioxide and sulfur dioxide capture from flue gas and enhanced hydrogen production with in-situ carbon dioxide capture using high reactivity calcium and biomineral sorbents. [D] . Iyer, Mahesh V. 2006

机译：高温反应分离工艺，用于从烟道气中捕获二氧化碳和二氧化硫，并使用高反应性钙和生物矿物吸附剂进行原位捕获，从而提高了制氢量。
6. Challengesin the Greener Production of Formates/FormicAcid Methanol and DME by Heterogeneously Catalyzed CO2 Hydrogenation Processes [O] . Andrea Álvarez, Atul Bansode, Atsushi Urakawa, -1

机译：挑战性在格式/格式的绿色生产中非均相催化CO2加氢工艺制得的酸甲醇和DME
7. Study on CO_2 catalytic hydrogenation For methanol synthesis [O] . 李基涛, 张伟德, 区泽棠 1998

机译：CO_2催化加氢合成甲醇的研究

Methanol from CO_2 by Organo-Cocatalysis: CO_2 Capture and Hydrogenation in One Process Step

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