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On the modeling of one-dimensional membrane reactors: Application to hydrogen production in fixed packed bed

机译:关于一维膜反应器的建模:在固定填充床制氢中的应用

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摘要

Hydrogen production by steam-methane reforming in membrane-assisted reactors has attracted substantial interest over the years. A variety of models for membrane-assisted reactors have been developed and suggested in the literature. In particular, examining the membrane models applied to the fixed packed bed reactor concept, there is no consensus or guidelines in the literature regarding the formulation of the heat balances (in terms of temperature). Thus, in the present study, different mathematical models for a fixed packed bed reactor with an integrated membrane have been compared in order to elucidate the effects of different model assumptions formulating the heat balance. The model formulations were examined by application to the steam-methane reforming process with hydrogen removal. The main findings of the present theoretical study are:
机译:多年来,在膜辅助反应器中通过蒸汽-甲烷重整制氢已经引起了人们的极大兴趣。已经开发了多种膜辅助反应器模型,并在文献中提出了建议。特别地,检查应用于固定填充床反应器概念的膜模型,在文献中关于热平衡的制定(就温度而言)没有共识或指南。因此,在本研究中,已比较了带有集成膜的固定填充床反应器的不同数学模型,以便阐明制定热平衡的不同模型假设的影响。通过将其应用于去除氢气的蒸汽-甲烷重整过程中,检验了模型配方。本理论研究的主要发现是:

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