Hydrodechlorination of Carbon Tetrachloride and 1,2-Dichloroethane on Palladium Nanoparticles Supported on Metal Fluorides

Machynskyy Ostap; Srebowata Anna; Kemnitz Erhard; Karpinski Zbigniew

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Hydrodechlorination of Carbon Tetrachloride and 1,2-Dichloroethane on Palladium Nanoparticles Supported on Metal Fluorides

机译：金属氟化物负载的钯纳米粒子对四氯化碳和1,2-二氯乙烷的加氢脱氯

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Catalytic activity of palladium supported on strongly acidic aluminum fluoride or on much less acidic magnesium fluoride has been the subject of current research. Both catalysts were synthesized by non-aqueous sol-gel method with subsequent two-stage activation: post-fluorination and reduction. The catalytic behavior of prepared Pd/HS-AlF3 and Pd/HS-MgF2 in the hydrodechlorination reactions of chlorinated hydrocarbons was investigated. It was found that differences in support acidity and catalyst's activation protocol strongly effect the catalytic performance.

机译：负载在强酸性氟化铝或弱酸性氟化镁上的钯的催化活性一直是当前研究的主题。两种催化剂均通过非水溶胶-凝胶法合成，并随后进行两步活化：后氟化和还原。研究了制备的Pd / HS-AlF3和Pd / HS-MgF2在氯代烃加氢脱氯反应中的催化行为。发现载体酸度和催化剂活化方案的差异强烈影响催化性能。

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《International journal of green energy》 |2015年第12期|780-786|共7页
作者
Machynskyy Ostap; Srebowata Anna; Kemnitz Erhard; Karpinski Zbigniew;
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作者单位

Polish Acad Sci, Inst Phys Chem, PL-01224 Warsaw, Poland;

Polish Acad Sci, Inst Phys Chem, PL-01224 Warsaw, Poland;

Humboldt Univ, Inst Chem, D-10099 Berlin, Germany;

Polish Acad Sci, Inst Phys Chem, PL-01224 Warsaw, Poland|Cardinal Stefan Wyszynski Univ, Fac Math & Nat Sci, Sch Sci, Warsaw, Poland;

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Nanoscopic aluminum fluoride and magnesium fluoride; Supported Pd nanoparticles; Hydrodechlorination of carbon tetrachloride and 1,2-dichloroethane;

机译：纳米级氟化铝和氟化镁;负载的钯纳米粒子;四氯化碳和1,2-二氯乙烷的加氢脱氯;

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专利

1. Active carbon-supported nickel-palladium catalysts for hydrodechlorination of 1,2-dichloroethane and 1,1,2-trichloroethene [J] . Kaminska I. I., Srebowata A. Research on Chemical Intermediates . 2015,第12期

机译：活性炭负载的镍钯催化剂用于1,2-二氯乙烷和1,1,2-三氯乙烯的加氢脱氯
2. Hydrodechlorination of 1,2-dichloroethane on active carbon supported palladium-nickel catalysts [J] . Anna Srgbowata, Wojciech Juszczyk, Zbigniew Kaszkur Catalysis Today . 2007,第1a2期

机译：活性炭负载钯镍催化剂上1,2-二氯乙烷的加氢脱氯
3. Hydrodechlorination over Pd-Pt/Al_2O_3 catalysts A comparative study of chlorine removal from dichlorodifluoromethane,carbon tetrachloride and 1,2-dichloroethane [J] . M.Legawiec-Jarzyna, A.Srebowata, W.Juszczyk Applied Catalysis, A. General: An International Journal Devoted to Catalytic Science and Its Applications . 2004,第1a2期

机译：Pd-Pt / Al_2O_3催化剂上的加氢脱氯从二氯二氟甲烷，四氯化碳和1,2-二氯乙烷中脱氯的比较研究
4. Multi-wall Carbon Nanotubes as a Support for Platinum Catalysts for the Hydrodechlorination of Carbon Tetrachloride and Dichlorodifluoromethane [C] . Magdalena Bonarowska, Kuan-Nan Lin, Marta Legawiec-Jarzyna, European Materials Research Society Fall Meeting . 2007

机译：多壁碳纳米管作为铂催化剂的载体四氯化碳和二氯二氟甲烷的铂催化剂
5. Selective hydrogenation of acetylene and hydrodechlorination of 1,2-dichloroethane over palladium bimetallic catalysts. [D] . Arsenault, Sarah. 2003

机译：在钯双金属催化剂上乙炔的选择性加氢和1,2-二氯乙烷的加氢脱氯。
6. Dehydrogenation of Ethylene on Supported Palladium Nanoparticles: A Double View from Metal and Hydrocarbon Sides [O] . Oleg A. Usoltsev, Anna Yu. Pnevskaya, Elizaveta G. Kamyshova, 2020

机译：负载钯纳米颗粒对乙烯的脱氢：金属和烃侧的双视图
7. Active carbon-supported nickel–palladium catalysts for hydrodechlorination of 1,2-dichloroethane and 1,1,2-trichloroethene [O] . 2015

机译：活性炭负载的镍钯催化剂，用于1,2-二氯乙烷和1,1,2-三氯乙烯的加氢脱氯
8. Health Advisories for 25 Organics (Including Acrylamide, Benzene, Carbon Tetrachloride, Chlorobenzene, Dichlorobenzene(s), 1,2-Dichloroethane, 1,1-Dichloroethylene, Cis-1,2-Dichloroethylene, Trans-1,2-Dichloroethylene, Dichloromethane, P-Dioxane, Dioxin, Epichlorohydrin, Ethylbeneze, Ethylene Glycol, Hexachlorobenezene, Hexane, Methyl Ethyl Ketone, Styrene, Tetrachloroethylene, Toluene, 1,1,1-Trichloroethane, Trichloroethylene, Vinyl Chloride, Xylenes) (RE-ANNOUNCEMENT of PB87-206306 - see notes field for explanation) [R] . 1987

机译：25种有机物的健康咨询（包括丙烯酰胺，苯，四氯化碳，氯苯，二氯苯，1,2-二氯乙烷，1,1-二氯乙烯，顺-1,2-二氯乙烯，反式-1,2-二氯乙烯，二氯甲烷），对二恶烷，二恶英，环氧氯丙烷，乙基苯乙烯，乙二醇，六氯苯，己烷，甲基乙基酮，苯乙烯，四氯乙烯，甲苯，1,1,1-三氯乙烷，三氯乙烯，氯乙烯，二甲苯）（pB87-的重新公告） 206306 - 请参阅备注字段以获取解释）

Hydrodechlorination of Carbon Tetrachloride and 1,2-Dichloroethane on Palladium Nanoparticles Supported on Metal Fluorides

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