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Intermixing-driven scenario for the growth of nanowires on (110) metal surfaces

机译:在(110)金属表面上生长纳米线的混合驱动方案

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摘要

The growth scenario of monatomic wires on fee (110) metal surfaces via intermixing of deposited and substrate atoms is reported. We present theoretical investigation of self-assembly of one-dimensional nano-structures during thermal deposition of Fe and Co atoms on Pd(110) in the submonolayer regime. Calculations performed by means of density-functional theory demonstrate that deposited atoms incorporate into the topmost substrate layer. Kinetic Monte Carlo simulations based on ab initio calculated diffusion barriers of relevant atomic processes indicate that surface diffusion of expelled atoms is responsible for growth of atomic wires consisting mainly of Pd atoms.
机译:报告了单原子线通过沉积原子和基底原子的混合在金属(110)上生长的情景。我们目前在亚单分子层体系中在Pd(110)上热沉积Fe和Co原子时一维纳米结构自组装的理论研究。借助密度泛函理论进行的计算表明,沉积的原子并入了最顶层的衬底层。基于从头计算的相关原子过程的扩散势垒的动力学蒙特卡洛模拟表明,被排出原子的表面扩散是主要由Pd原子组成的原子线生长的原因。

著录项

  • 来源
    《Physical review》 |2009年第15期|751-755|共5页
  • 作者单位

    Faculty of Physics, Moscow State University, 119899 Moscow, Russia;

    Fachbereich Phvsik, Martin-Luther-Universitaet, Halle-Wittenberg, Friedemann-Bach-Platz 6, D-06099 Halle, Germany;

    Max-Planck-Institute fuer Mikrostrukturphysik, Weinberg 2, D-06120 Halle, Germany;

    Max-Planck-Institute fuer Mikrostrukturphysik, Weinberg 2, D-06120 Halle, Germany;

    Fachbereich Phvsik, Martin-Luther-Universitaet, Halle-Wittenberg, Friedemann-Bach-Platz 6, D-06099 Halle, Germany;

    Faculty of Physics, Moscow State University, 119899 Moscow, Russia;

    Max-Planck-Institute fuer Mikrostrukturphysik, Weinberg 2, D-06120 Halle, Germany;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    self-assembly; quantum wires;

    机译:自组装;量子线;

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