Dynamic combinatorial synthesis of a catenane based on donor-acceptor interactions in water

Ho Yu Au-Yeung; G. Dan Pantos; Jeremy K. M. Sanders

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Dynamic combinatorial synthesis of a catenane based on donor-acceptor interactions in water

机译：基于水中供体-受体相互作用的链烷烃的动态组合合成

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A new type of neutral donor-acceptor [2]-catenane, containing both complementary units in the same ring was synthesized from a dynamic combinatorial library in water. The yield of the water soluble [2]-catenane is enhanced by increasing either building-block concentrations or ionic strength, or by the addition of an electron-rich template. NMR spectroscopy demonstrates that the template is intercalated between the 2 electron-deficient naph-thalenediimide units of the catenane.

机译：从水中的动态组合库合成了一种新型的中性供体-受体[2]-联烷，在同一环中包含两个互补单元。通过增加结构单元浓度或离子强度，或通过添加富电子模板，可提高水溶性[2]-联烷烃的收率。 NMR光谱表明，该模板插入了链烷烃的两个缺电子的萘-次烷基二酰亚胺单元之间。

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《Proceedings of the National Academy of Sciences of the United States of America》 |2009年第26期|10466-10470|共5页
作者
Ho Yu Au-Yeung; G. Dan Pantos; Jeremy K. M. Sanders;
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作者单位

University Chemical Laboratory, University of Cambridge, Lensfield Road, Cambridge CB2 1EW, United Kingdom;

University Chemical Laboratory, University of Cambridge, Lensfield Road, Cambridge CB2 1EW, United Kingdom;

University Chemical Laboratory, University of Cambridge, Lensfield Road, Cambridge CB2 1EW, United Kingdom;

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收录信息美国《科学引文索引》(SCI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
原文格式 PDF
正文语种 eng
中图分类
关键词
dynamic combinatorial chemistry; molecular recognition;

机译：动态组合化学分子识别;

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专利

1. Dynamic combinatorial donor-acceptor catenanes in water: Access to unconventional and unexpected structures [J] . Au-Yeung H.Y., Panto? G.D., Sanders J.K.M. The Journal of Organic Chemistry . 2011,第5期

机译：水中动态的组合供体-受体链烯：进入非常规和意外结构的通道
2. Exploring the Formation Pathways of Donor-Acceptor Catenanes in Aqueous Dynamic Combinatorial Libraries [J] . Fabien B. L. Cougnon, Ho Yu Au-Yeung, G. Dan Pantoş, Journal of the American Chemical Society . 2011,第9期

机译：探索水性动态组合图书馆中供体-受体链的形成途径。
3. Amplifying Different [2]Catenanes in an Aqueous Donor-Acceptor Dynamic Combinatorial Library [J] . Ho Yu Au-Yeung, G. Dan Pantos, Jeremy K. M. Sanders Journal of the American Chemical Society . 2009,第44期

机译：扩增供体-受体动态组合库中的不同[2]儿茶酚
4. Diffusion of Water in Silicalite by Molecular Dynamics Simulations: Ab Initio based interactions [C] . C. Bussai, S. Hannongbua, S. Fritzsche, Impact of Zeolites and Other Porous Materials on the New Technologies at the Beginning of the New Millennium . 2002

机译：水在硅藻土中扩散的分子动力学模拟：基于从头算的相互作用
5. I. Synthesis and dynamic studies of bifunctional compounds having potential intramolecular interactions. II. Controlled release antifouling coatings: Approaches to controlled release of gamma-decanolactone and 2-hexanoylfuran into seawater. [D] . West, Craig Anthony. 1995

机译：I.具有潜在分子内相互作用的双功能化合物的合成和动力学研究。二。控释防污涂料：γ-癸内酯和2-己基呋喃向海水中的控制释放方法。
6. Molecular Recognition and Self-Assembly Special Feature: Dynamic combinatorial synthesis of a catenane based on donor–acceptor interactions in water [O] . Ho Yu Au-Yeung, G. Dan Pantoş, Jeremy K. M. Sanders 2009

机译：分子识别和自组装特征：基于水中供体-受体相互作用的链烷烃的动态组合合成
7. Molecular recognition and self-assembly special feature: Dynamic combinatorial synthesis of a catenane based on donor-acceptor interactions in water [O] . Au-Yeung, H Y, Pantoș, G Dan, Sanders, J K 2009

机译：分子识别和自组装特征：基于水中供体-受体相互作用的链烷烃的动态组合合成

Dynamic combinatorial synthesis of a catenane based on donor-acceptor interactions in water

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