Copper(I) Zeolites as Heterogeneous and Ligand-Free Catalysts: [3+2] Cycloaddition of Azomethine Imines

Murielle Keller; Abdelkarim Sani Souna Sido; Patrick Pale; Jean Sommer

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Copper(I) Zeolites as Heterogeneous and Ligand-Free Catalysts: [3+2] Cycloaddition of Azomethine Imines

机译：铜（I）沸石作为多相和无配体催化剂：偶氮甲亚胺的[3 + 2]环加成反应

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Copper(I)-exchanged zeolites were used as heterogeneous ligand-free catalysts for [3+2] cycloaddition of azomethine ylides, which allows versatile, efficient, and highly regioselective synthesis of pyrazolone derivatives. These cheap and easy-to-prepare catalysts exhibit wide scope and compatibility with functional groups. They are very simple to use, easy to remove (by simple filtration), and recyclable (up to six times without loss of activity).

机译：铜（I）交换的沸石用作偶氮次甲基的[3 + 2]环加成反应的无均相无配体催化剂，可实现吡唑啉酮衍生物的通用，高效和高度区域选择性合成。这些廉价且易于制备的催化剂表现出宽范围和与官能团的相容性。它们非常易于使用，易于去除（通过简单过滤）和可回收利用（最多可回收六次，而不会损失活性）。

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来源
《Chemistry: A European journal》 |2009年第12期|共8页
作者
Murielle Keller; Abdelkarim Sani Souna Sido; Patrick Pale; Jean Sommer;
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原文格式 PDF
正文语种 eng
中图分类应用化学;
关键词
click chemistry; copper; cycloaddition; heterogeneous catalysis; zeolites;

机译：点击化学;铜;环加成;非均相催化;沸石;

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1. Copper(I) Zeolites as Heterogeneous and Ligand-Free Catalysts: [3+2] Cycloaddition of Azomethine Imines [J] . Murielle Keller, Abdelkarim Sani Souna Sido, Patrick Pale, Chemistry: A European journal . 2009,第12期

机译：铜（I）沸石作为多相和无配体催化剂：偶氮甲亚胺的[3 + 2]环加成反应
2. [3+2] Cycloaddition of Azomethine Imines and Alkynes with Copper(I) Zeolites [J] . M. KELLER, A. S. S. SIDO, P. PALE, Synfacts: highlights in current synthetic organic chemistry . 2009,第5期

机译：[3 + 2]杂多亚胺亚胺和炔烃与铜（I）沸石的环加成反应
3. Natrolite zeolite supported copper nanoparticles as an efficient heterogeneous catalyst for the 1,3-diploar cycloaddition and cyanation of aryl iodides under ligand-free conditions [J] . Nasrollahzadeh Mahmoud, Sajadi S. Mohammad, Rostami-Vartooni Akbar, Journal of Colloid and Interface Science . 2015,第Null期

机译：钠沸石沸石负载的铜纳米颗粒作为无配位条件下芳基碘化物的1,3-二齿环加成和氰化的高效多相催化剂
4. 3+2 Cycloadditions of Aromatic Azomethine Imines with Allenoates [C] . Lei Zhang, Chengfeng Jing, Honglei Liu, Proceedings of 4th international symposium on pesticides and environmental safety amp; 5th pan Pacific confernce on pesticide science amp; 8th international workshop on crop protection chemistry and regulatory harmonization . 2012

机译：3 + 2芳香族甲亚胺亚胺与烯丙酸酯的环加成
5. I. Completion of the synthesis of Kopsia lapidilecta alkaloid (+/-)-lapidilectine B. II. Synthesis of 1-azabicyclo[n.3.0]alkanes via [3+2] cycloadditions of nonstabilized azomethine ylides [D] . Stoy, Patrick 2004

机译：I.完成了Kopsia lapidilecta生物碱（+/-）-lapidilectine的合成B. II。通过不稳定的偶氮甲亚胺的[3 + 2]环加成反应合成1-氮杂双环[n.3.0]烷烃
6. Synthesis of Non-Racemic Pyrazolines and Pyrazolidines by 3+2 Cycloadditions of Azomethine Imines [O] . Franc Požgan, Hamad Al Mamari, Uroš Grošelj, 2018

机译：3 + 2苯甲亚胺亚胺的环加成反应合成非放射性吡唑啉和吡唑烷
7. Kinetic resolutions of azomethine imines via copper-catalyzed 3+2 cycloadditions [O] . C. Wade Downey, Gregory C. Fu 2014

机译：通过铜催化的3 + 2环加成反应得到甲亚胺亚胺的动力学分辨率

Copper(I) Zeolites as Heterogeneous and Ligand-Free Catalysts: [3+2] Cycloaddition of Azomethine Imines

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