Oxidative coupling of aromatic substrates with alkynes and alkenes under Rhodium Catalysis

Satoh T.; Miura M.

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Oxidative coupling of aromatic substrates with alkynes and alkenes under Rhodium Catalysis

机译：铑催化下芳香族底物与炔烃和烯烃的氧化偶联

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摘要

Aromatic substrates with oxygen-and nitrogen-containing substituents undergo oxidative coupling with alkynes and alkenes under rhodium catalysis through re-gioselective C-H bond cleavage. Coordination of the sub-stituents to the rhodium center is the key to activate the C-H bonds effectively. Various fused-ring systems can be constructed through these reactions.

机译：具有含氧和氮取代基的芳族底物在铑催化下，通过区域选择性C-H键断裂，与炔烃和烯烃进行氧化偶联。取代基与铑中心的配位是有效激活C-H键的关键。通过这些反应可以构建各种稠环系统。

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《Chemistry: A European journal》 |2010年第37期|共11页
作者
Satoh T.; Miura M.;
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正文语种 eng
中图分类应用化学;
关键词
C-H activation; Fused-ring systems; Homogeneous catalysis; Oxidative coupling; Rhodium;

机译：碳氢活化稠环体系均相催化氧化偶联铑;

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专利

1. Oxidative coupling of aromatic substrates with alkynes and alkenes under Rhodium Catalysis [J] . Satoh T., Miura M. Chemistry: A European journal . 2010,第37期

机译：铑催化下芳香族底物与炔烃和烯烃的氧化偶联
2. Rhodium(III)-Catalyzed Oxidative Coupling of N-Phenylindole-3-carboxylic Acids with Alkenes and Alkynes via C4–H and C2–H/C2′–H Bond Cleavage [J] . Takeshi Okada, Asumi Sakai, Tomoaki Hinoue, The Journal of Organic Chemistry . 2018,第10期

机译：通过C4-H和C2-H / C2'-H键裂解铑（III）与烯基吲哚-3-羧酸的催化氧化偶联 n℃和炔基-3-羧酸
3. Synthesis of Functionalized r-Pyrone and Butenolide Derivatives by Rhodium-Catalyzed Oxidative Coupling of Substituted Acrylic Acids with Alkynes and Alkenes [J] . Satoshi Mochida, Koji Hirano, Tetsuya Satoh, The Journal of Organic Chemistry . 2009,第16期

机译：铑催化的丙烯酸与炔烃和烯烃的氧化偶联偶联合成功能化的r-吡咯酮和丁烯内酯衍生物
4. Rhodium(III)-Catalyzed Oxidative Coupling of Isoxazolyl-4- carboxylic acids with Alkynes: Oxidants Control the Formation of Pyranoisoxazolones and Isoquinolines [C] . Somaraju Yugandar, Hiroyuki Nakamura 日本化学会春季年会講演予稿集 . 2018

机译：铑（III） - 丙基唑氧基-4-羧酸与炔烃的催化偶联：氧化剂控制吡喃异恶唑啉和异喹啉的形成
5. Heterocycle Synthesis via Titanium-Mediated Cross-Coupling of Imines with Alkenes and Alkynes [D] . Chen, Ming Zhu 2012

机译：钛介导的亚胺与烯烃和炔烃的交叉偶联合成杂环
6. Asymmetric Catalysis Special Feature Part I: Rhodium-catalyzed asymmetric ring opening reactions of oxabicyclic alkenes: Catalyst and substrate studies leading to a mechanistic working model [O] . Mark Lautens, Keith Fagnou 2004

机译：不对称催化的特殊功能（第一部分）：铑催化的氧杂双环烯烃的不对称开环反应：催化剂和底物的研究产生了一种机械的工作模型
7. Rhodium-Catalyzed Intermolecular Chelation Controlled Alkene and Alkyne Hydroacylation: Synthetic Scope of b-S-Substituted Aldehyde Substrates [O] . -1

机译：铑催化的分子间螯合控制烯烃和炔烃：B-S取代醛底物的合成范围

Oxidative coupling of aromatic substrates with alkynes and alkenes under Rhodium Catalysis

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