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A quantum electrodynamical treatment of second harmonic generation through phase conjugate six-wave mixing: Polarization analysis

机译:相位共轭六波混频产生二次谐波的量子电动力学处理:极化分析

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摘要

The theory underlying a six-wave mixing experiment is developed using the methods of molecular quantum electrodynamics. This general theory allows the intensity of the second harmonic radiation generated by the six-wave process to be found for arbitrary arrangements of the generating laser beams. Several different polarization geometries are treated in detail, and comparison is made to experiments performed using near-resonant conditions. The agreement is good in all cases and allows detailed information pertaining to the six-wave tensor to be extracted. The information thus obtained provides evidence of a marked departure from Kleinman symmetry. (C) 1998 American Institute of Physics. [S0021-9606(98)01948-5]. [References: 26]
机译:使用分子量子电动力学方法开发了六波混合实验的基础理论。该一般理论允许对于产生的激光束的任意布置找到由六波过程产生的二次谐波辐射的强度。详细介绍了几种不同的极化几何,并与使用近共振条件进行的实验进行了比较。该协议在所有情况下都是好的,并允许提取与六波张量有关的详细信息。这样获得的信息提供了明显偏离克莱曼对称性的证据。 (C)1998美国物理研究所。 [S0021-9606(98)01948-5]。 [参考:26]

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