SC_nS Linear Chain Production by Direct Laser Ablation

Andrei Burnin; Joseph J. BelBruno

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SC_nS Linear Chain Production by Direct Laser Ablation

机译：通过直接激光烧蚀生产SC_nS线性链

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Cumulenic polycarbons SC_nS (n = 2-27) were generated by laser ablation of mixtures of elemental carbon and sulfur. The resulting molecules were analyzed in a time-of-flight mass spectrometer. The spectra exhibited ideal odd/even intensity alternation attributed to their relative stability and the formation mechanism of the clusters. The structures and energies of the neutral and charged carbon chains capped with two sulfur atoms were also studied by density functional theory. The computational results were consistent with the experimental observations. Evidence of sulfur poisoning of fullerene formation was observed and explained in terms of one of the existing models for fullerene formation and growth.

机译：通过对元素碳和硫的混合物进行激光烧蚀，生成了立方型聚碳酸酯SC_nS（n = 2-27）。在飞行时间质谱仪中分析所得分子。光谱表现出理想的奇/偶强度交替，这归因于它们的相对稳定性和团簇的形成机理。还通过密度泛函理论研究了被两个硫原子覆盖的中性和带电碳链的结构和能量。计算结果与实验结果一致。观察到并根据现有的富勒烯形成和生长模型之一解释了富勒烯形成的硫中毒证据。

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《The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory》 |2003年第45期|共7页
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Andrei Burnin; Joseph J. BelBruno;
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正文语种 eng
中图分类物理化学（理论化学）、化学物理学;
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1. SC_nS Linear Chain Production by Direct Laser Ablation [J] . Andrei Burnin, Joseph J. BelBruno The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory . 2003,第45期

机译：通过直接激光烧蚀生产SC_nS线性链
2. Direct synthesis of size-tailored bimetallic Ag/Au nano-spheres and nano-chains with controllable compositions by laser ablation of silver plate in HAuCl4 solution [J] . Ming Chen, DaMeng Wang, XiangDong Liu RSC Advances . 2016,第12期

机译：通过HauCl4溶液中的银板的激光烧蚀直接合成尺寸定制的双金属Ag / Au纳米球和纳米链
3. The effects of liquid environments on the optical properties of linear carbon chains prepared by laser ablation generated plasmas [J] . G. Forte, L.DUrso, E.Fazio, Applied Surface Science . 2013,第maya1期

机译：液体环境对通过激光烧蚀产生的等离子体制备的线性碳链的光学性质的影响
4. Interaction between linear carbon chains and metal NPs preparedby laser ablation in water [C] . G.C. Messina, L. DUrso, E. Messina, EOS conference on laser ablation and nanoparticle generation in liquids 2010 . 2010

机译：水中激光烧蚀制备线性碳链与金属纳米粒子之间的相互作用
5. Spectroscopic studies of long carbon and silicon -carbon chains produced by laser ablation. [D] . Ding, Xiande (Sam). 2000

机译：激光烧蚀产生的长碳链和硅碳链的光谱学研究。
6. Randomized clinical trial of endovenous laser ablation versus direct and indirect radiofrequency ablation for the treatment of great saphenous varicose veins [O] . S. A. S. Hamann, L. Timmer‐de Mik, W. M. Fritschy, -1

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7. Correction for ‘Direct analysis of dried blood spots by femtosecond-laser ablation-inductively coupled plasma-mass spectrometry. Feasibility of split-flow laser ablation for simultaneous trace element and isotopic analysis’ by M. Aramendía et al., J. Anal. At. Spectrom., 2015, DOI: 10.1039/c4ja00313f. [O] . Aramendía, M., Rello, L., Berail, S., 2015

机译：通过飞秒激光消融-电感耦合等离子体质谱法对“直接分析干血斑进行校正”。 M.Aramendía等人，J。Anal。着，用分流激光烧蚀同时进行痕量元素和同位素分析的可行性。在。光谱。，2015，DOI：10.1039 / c4ja00313f。

SC_nS Linear Chain Production by Direct Laser Ablation

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