Scaling of Fluorescence Stokes Shift and Superradiance Coherence Size in Disordered Molecular Aggregates

Vladimir Chernyak; Torsten Meier; Eugene Tsiper; Shaul Mukamel

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Scaling of Fluorescence Stokes Shift and Superradiance Coherence Size in Disordered Molecular Aggregates

机译：无序分子聚集体中的荧光斯托克斯位移和超辐射相干大小的缩放比例。

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Fluorescence line shapes and cooperative spontaneous emission in disordered one-dimensional molecular aggregates are calculated using closed expression derived by applying the method of optimal fluctuation. A simple scaling relation L_s approx #omega#_s~(-1/2) is established between the low temperature disorder-induced Stokes shift #omega#_s and the superradiance enhancement factor L_s. Scaling of the Stokes shift with aggregate size, and the time-dependent Stokes shift are discussed as well. Excellent agreement is obtained with numerical simulations.

机译：利用最优波动法导出的封闭表达式，计算了无序一维分子聚集体中的荧光线形状和协同自发发射。在低温紊乱引起的斯托克斯位移＃omega＃_s与超辐射增强因子L_s之间建立了简单的比例关系L_s约＃omega＃_s〜（-1/2）。还讨论了具有聚合大小的Stokes位移的缩放比例以及与时间有关的Stokes位移。通过数值模拟可以获得极好的一致性。

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《The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory》 |1999年第49期|共6页
作者
Vladimir Chernyak; Torsten Meier; Eugene Tsiper; Shaul Mukamel;
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正文语种 eng
中图分类物理化学（理论化学）、化学物理学;
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1. Scaling of Fluorescence Stokes Shift and Superradiance Coherence Size in Disordered Molecular Aggregates [J] . Vladimir Chernyak, Torsten Meier, Eugene Tsiper, The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory . 1999,第49期

机译：无序分子聚集体中的荧光斯托克斯位移和超辐射相干大小的缩放比例。
2. Finite size line broadening and superradiance of optical transitions in two dimensional long-range ordered molecular aggregates [J] . Müller M., Paulheim A., Eisfeld A., The Journal of Chemical Physics . 2013,第4期

机译：二维远距离有序分子聚集体的有限尺寸线展宽和光学跃迁的超辐射
3. Fully Integrated High-Speed Intravascular Optical Coherence Tomography/Near-Infrared Fluorescence Structural/Molecular Imaging In Vivo Using a Clinically Available Near-Infrared Fluorescence-Emitting Indocyanine Green to Detect Inflamed Lipid-Rich Atheromata in Coronary-Sized Vessels. [J] . Sunki, Lee, Min Woo, Circulation. Cardiovascular interventions . 2014,第4期

机译：完全集成的高速血管内光学相干断层扫描/近红外荧光结构/分子成像，使用临床可得的近红外发光吲哚菁绿在冠状血管中检测发炎的富含脂质的动脉瘤。
4. Superradiance and exciton dynamics in molecular aggregates [C] . Henk Fidder, Jacob Terpstra, Douwe A. Wiersma Intermational conference on laser applications in life sciences . 1994

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5. Coverage and interval length of Welch's and Yuen's procedures for shift in location and change in scale for (un)equal sample sizes [D] . Mends-Cole, Saydee Jonathan. 2006

机译：（不）相等样本量的Welch和Yuen程序的位置转移和规模变化的覆盖范围和间隔长度
6. Engineering of mCherry variants with long Stokes shift red-shifted fluorescence and low cytotoxicity [O] . Yi Shen, Yingche Chen, Jiahui Wu, -1

机译：具有长斯托克斯频移红移荧光和低细胞毒性的mCherry变体工程
7. Scaling of Fluorescence Stokes Shift and Superradiance Coherence Size in Disordered Molecular Aggregates [O] . Vladimir Chernyak, Torsten Meier, Eugene Tsiper, 1999

机译：无序分子聚集体中荧光斯托克斯位移和超辐射相干尺寸的缩放

Scaling of Fluorescence Stokes Shift and Superradiance Coherence Size in Disordered Molecular Aggregates

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