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首页> 外文期刊>The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory >Transformations in Crystalline Ammonium Nickel Tutton Salt Induced by Infrared Hole Burning
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Transformations in Crystalline Ammonium Nickel Tutton Salt Induced by Infrared Hole Burning

机译：红外孔燃烧引起的结晶态铵态镍镍顿盐的转变

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摘要

The title compound doped with a small amount of deuterium shows infrared bands due to the N-D and O-D stretching vibrations. When one of the N-D bands is irradiated with an infrared laser, holes and antiholes are produced. The pattern of these holes/anti-holes depends on the irradiation time. A ten-minute irradiation produces holes/anti-holes in the N-D bands only. A ten-second irradiation produes holes/antiholes in the O-D bands as well. The features produced by the ten-second irradiation decay during the longer irradiation. Thus, the durning and decay kinetics of the Tutton salts involve processes that occur on at least two time scales.
机译：掺杂有少量氘的标题化合物由于N-D和O-D拉伸振动而显示红外波段。当用红外激光照射N-D波段之一时，会产生空穴和反空穴。这些孔/防孔的图案取决于照射时间。十分钟的照射仅在N-D波段产生空穴/反空穴。十秒钟的照射也会在O-D波段产生空穴/反空穴。十秒辐照产生的特征在更长的辐照期间会衰减。因此，图顿盐的盐析动力学和衰减动力学涉及至少在两个时间尺度上发生的过程。

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