EFFECT OF MECHANICOCHEMICAL TREATMENT ON THE ACTIVITY OF K2PdCl4 IN THE HETEROGENEOUS CATALYTIC HYDROCHLORINATION OF ACETYLENE

S. A. Mitchenko; T. V. Krasnyakova; I. V. Zhikharev

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EFFECT OF MECHANICOCHEMICAL TREATMENT ON THE ACTIVITY OF K2PdCl4 IN THE HETEROGENEOUS CATALYTIC HYDROCHLORINATION OF ACETYLENE

机译：机械化学处理对乙炔非均相催化加氢氯化过程中K2PdCl4活性的影响

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摘要

A heterogeneous catalyst for the hydrochlorination of acetylene using gaseous HCl was obtained by prior mechanical activation of K2PdCl4 powder in an atmosphere of acetylene or propylene. Active sites are formed during the mechanical treatment in the surface layers of the catalyst, which are Pd(II) complexes with a coordination vacancy.

机译：通过先在乙炔或丙烯气氛中对K2PdCl4粉末进行机械活化，可获得使用气态HCl进行乙炔氢氯化的非均相催化剂。在机械处理过程中，在催化剂表面层中形成了活性位点，这些位点是具有配位空位的Pd（II）配合物。

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《Theoretical and Experimental Chemistry》 |2010年第1期|共7页
作者
S. A. Mitchenko; T. V. Krasnyakova; I. V. Zhikharev;
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正文语种 eng
中图分类化学;
关键词
acetylene; hydrochlorination; heterogeneous catalysis; active sites; palladium(II) complexes; mechanical activation;

机译：乙炔;氯化氢;多相催化;活性位点;钯（II）配合物;机械活化;

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1. EFFECT OF MECHANICOCHEMICAL TREATMENT ON THE ACTIVITY OF K2PdCl4 IN THE HETEROGENEOUS CATALYTIC HYDROCHLORINATION OF ACETYLENE [J] . S. A. Mitchenko, T. V. Krasnyakova, I. V. Zhikharev Theoretical and Experimental Chemistry . 2010,第1期

机译：机械化学处理对乙炔非均相催化加氢氯化过程中K2PdCl4活性的影响
2. CATALYTIC HYDROCHLORINATION OF ACETYLENE ON MECHANOCHEMICALLY-ACTIVATED K2PdCl4 [J] . S. A. Mitchenko, T. V. Krasnyakova, I. V. Zhikharev Theoretical and Experimental Chemistry . 2008,第5期

机译：机械活化的K2PdCl4催化乙炔加氢氯化
3. Estimates of the catalytic efficiency of a heterogeneous catalyst for acetylene hydrochlorination on the surface of mechanically activated K2PtCl6 salt [J] . Mitchenko SA, Khomutov EV, Shubin AA, Kinetics and catalysis . 2004,第3期

机译：机械活化的K2PtCl6盐表面乙炔盐酸盐多相催化剂催化效率的估算
4. Simulation Analysis of Fixed Bed Reactor for Au-Cu Non-mercury Catalytic Acetylene Hydrochlorination [C] . Lei Wang, Ben-xian Shen, Ruo-fan Ren, International Conference on Mechanical Materials and Manufacturing Engineering . 2014

机译：Au-Cu非汞催化乙炔氢氯化固定床反应器的仿真分析
5. Investigation of Oxidized Carbon Supported Au Catalysts Synthesized Via Strong Electrostatic Adsorption of Au(en)2Cl3 for the Hydrochlorination of Acetylene to Vinyl Chloride Monomer [D] . ?Noble, Sean Reginald 2020

机译：通过强大的静电吸附于Au（Zh）2Cl3的乙炔氢氯化对氯乙烯单体的乙酰氯化氢氯化的氧化碳负载的Au催化剂的研究
6. Effect of various g-C3N4 precursors on the catalytic performance of alkylorganotin-based catalysts in acetylene hydrochlorination [O] . Yibo Wu, Fuxiang LI, Jianwei XUE, 2020

机译：各种G-C3N4前体对乙炔氢氯化铝基催化剂催化性能的影响
7. Self- regeneration of Au/CeO2 based catalysts with enhanced activity and ultra-stability for acetylene hydrochlorination [O] . Lin Ye, Xinping Duan, Simson Wu, 2019

机译：基于Au / CeO2的催化剂的自再生，具有增强的活性和超稳定性对乙炔氢氯化物

EFFECT OF MECHANICOCHEMICAL TREATMENT ON THE ACTIVITY OF K2PdCl4 IN THE HETEROGENEOUS CATALYTIC HYDROCHLORINATION OF ACETYLENE

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