Photooxidation of methane to methanol by perrhenate in water under ambient conditions

Kunkely H.; Vogler A.

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Photooxidation of methane to methanol by perrhenate in water under ambient conditions

机译：在环境条件下，水中高water酸盐将甲烷光氧化为甲醇

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The oxidation of methane to methanol takes place selectively by the photolysis of perrhenate in aqueous solution in the presence of methane. This photoreaction is formally an oxygen atom transfer. Because the reoxidation of the reduced perrhenate is accomplished with hydrogen peroxide the overall process can be viewed as photocatalytic oxidation of methane to methanol: CH_4 +H_2O_2 ? CH_3OH+ H_2O.

机译：甲烷氧化为甲醇是通过在甲烷存在下水溶液中高r酸盐的光解选择性地进行的。这种光反应形式上是氧原子转移。因为还原的高hen酸盐的再氧化是用过氧化氢完成的，所以整个过程可以看成是甲烷将甲烷光催化氧化为甲醇的反应：CH_4 + H_2O_2？ CH_3OH + H_2O。

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《Zeitschrift fur Naturforschung, B. A Journal of Chemical Sciences》 |2013年第8期|共4页
作者
Kunkely H.; Vogler A.;
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原文格式 PDF
正文语种 eng
中图分类 54;
关键词
Catalysis; Methane; Photochemistry; Rhenium complexes;

机译：催化;甲烷;光化学;R配合物;

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1. Photooxidation of methane to methanol by perrhenate in water under ambient conditions [J] . Kunkely H., Vogler A. Zeitschrift fur Naturforschung, B. A Journal of Chemical Sciences . 2013,第8期

机译：在环境条件下，水中高water酸盐将甲烷光氧化为甲醇
2. Catalytic DBD plasma approach for methane partial oxidation to methanol under ambient conditions [J] . Chawdhury Piu, Ray Debjyoti, Vinodkumar T., Catalysis Today . 2019,第期

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3. Thermal and spectral characterization and stability of mixtures of ionic liquids [EMIM]Ac and [BMIM]Ac with ethanol, methanol, and water at ambient conditions and at elevated temperatures and pressures [J] . Williams Michael L., Holahan Scott P., McCorkill Mary E., Thermochimica Acta: An International Journal Concerned with the Broader Aspects of Thermochemistry and Its Applications to Chemical Problems . 2018,第期

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4. Direct conversion of methane to methanol over Copper-Exchanged Zeolites under mild conditions [C] . ZENG R., Li L., Shimizu T 化学工学会年会 . 2020

机译：在温和条件下将甲烷直接转化甲烷在铜交换沸石上的甲醇
5. Treatment of Cyanotoxins in Rivers and River Influenced Groundwater under Ambient and Softened pH Conditions. [D] . Neemann, Jeffrey John. 2016

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6. Solubility of Tris(hydroxymethyl)aminomethane in Water-Methanol Solvent Mixtures and Medium Effects in the Dissociation of the Protonated Base [O] . Paul Schindler, R. A. Robinson, Roger G. Bates 1968

机译：三（羟甲基）氨基甲烷在水-甲醇溶剂混合物中的溶解度和介质对质子化碱解离的影响
7. Highly selective oxidation of methane to methanol at ambient conditions by titanium dioxide-supported iron species [O] . Jijia Xie, Renxi Jin, Ang Li, 2018

机译：通过二氧化钛支持的铁物种在环境条件下高度选择性氧化甲烷至甲醇
8. Photooxidation of Groundwater Contaminants: Trichloroethylene, Trichloromethane,Dibromochloropropane and Benzene. A Critical Review [R] . Burrows, W. D. 1994

机译：地下水污染物的光氧化：三氯乙烯，三氯甲烷，二溴氯丙烷和苯。评论性评论

Photooxidation of methane to methanol by perrhenate in water under ambient conditions

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