Why the optimal ammonia synthesis catalyst is not the optimal ammonia decomposition catalyst

Astrid Boisen; Soren Dahl; Jens K.Norskov; Claus Hvud Christensen

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Why the optimal ammonia synthesis catalyst is not the optimal ammonia decomposition catalyst

机译：为什么最佳氨合成催化剂不是最佳氨分解催化剂

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Developments in ammonia synthesis have also made it possible to take a more rational approach to research on ammonia decomposition.It has been found that the optimal catalyst for ammonia synthesis is never the optimal catalyst for ammonia decomposition,which is almost counter-intuitive in catalysis research.The approach taken for ammonia synthesis/decomposition could be useful for many other systems and lead to a more rational development of new and improved catalysts and catalytic processes.

机译：氨合成技术的发展也使得采用更合理的方法进行氨分解研究成为可能。发现氨合成的最佳催化剂永远不会是氨分解的最佳催化剂，这在催化研究中几乎是违反直觉的。用于氨合成/分解的方法可能对许多其他系统有用，并导致更合理地开发新的和改良的催化剂和催化方法。

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《Journal of Catalysis》 |2005年第2期|共4页
作者
Astrid Boisen; Soren Dahl; Jens K.Norskov; Claus Hvud Christensen;
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正文语种 eng
中图分类高分子化学（高聚物）;
关键词
Ammonia decomposition; Ammonia synthesis; DFT; Heterogeneous catalysis; Kinetics;

机译：氨分解氨合成DFT非均相催化动力学;

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1. Why the optimal ammonia synthesis catalyst is not the optimal ammonia decomposition catalyst [J] . Astrid Boisen, Soren Dahl, Jens K.Norskov, Journal of Catalysis . 2005,第2期

机译：为什么最佳氨合成催化剂不是最佳氨分解催化剂
2. The effect of iron nanocrystallites’ size in catalysts for ammonia synthesis on nitriding reaction and catalytic ammonia decomposition [J] . Rafa? Pelka, Karolina Kie?basa, Walerian Arabczyk Open Chemistry . 2011,第2期

机译：氨合成催化剂中铁纳米晶尺寸对氮化反应和氨催化分解的影响
3. Ammonia Decomposition and Synthesis over Multinary Magnesioferrites: Promotional Effect of Ga on Fe Catalysts for the Decomposition Reaction [J] . ChemCatChem . 2017,第4期

机译：多元镁铁氧体氨分解和合成：Ga对分解反应的Fe催化剂的促进作用
4. Comparison of the activity of Ru-K/Sibunit catalysts in ammonia synthesis and decomposition [C] . D. A. Petrunin, V. A. Borisov, K. N. Iost, Oil and Gas Engineering . 2019

机译：Ru-K / SibUnit催化剂在氨合成和分解中的活性比较
5. High throughput investigation of supported catalysts for carbon oxides-free hydrogen production from ammonia decomposition. [D] . D'Addio, Elizabeth M. 2011

机译：高通量研究负载型催化剂用于氨分解产生无碳氧化物的氢气。
6. Material Discovery and High Throughput Exploration of Ru Based Catalysts for Low Temperature Ammonia Decomposition [O] . Katherine McCullough, Pei-Hua Chiang, Juan D. Jimenez, 2020

机译：钌基低温氨分解催化剂的材料发现和高通量探索
7. Ammonia Decomposition and Synthesis over Multinary Magnesioferrites: Promotional Effect of Ga on Fe Catalysts for the Decomposition Reaction [O] . Friedel Ortega K., Rein D., Lüttmann C., 2017

机译：多元磁性铁的氨分解与合成：Ga对Fe催化剂分解反应的促进作用

Why the optimal ammonia synthesis catalyst is not the optimal ammonia decomposition catalyst

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