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首页> 外文期刊>Journal of Geophysical Research. Biogeosciences >Emission inventory development and processing for the Seasonal Model for Regional Air Quality (SMRAQ) project
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Emission inventory development and processing for the Seasonal Model for Regional Air Quality (SMRAQ) project

机译:区域空气质量季节性模型(SMRAQ)项目的排放清单开发和处理

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This paper describes the experiences and insights gained from inventory preparation and emissions processing for the Seasonal Model for Regional Air Quality (SMRAQ) project. The emission inventory was derived from the 1990 and 1995 Ozone Transport Assessment Group (OTAG) inventories. Here we outline the emissions processing strategy used for the May-to-September simulation, summarize the inventory characteristics and corrections made on the OTAG inventories, and describe the quality assurance steps taken as part of the processing. We then provide spatial maps and daily total time series charts of the hourly, gridded emissions of nitrogen oxides (NOx), reactive organic gases (ROG), and carbon monoxide (CO). Large peaks from electric utility point sources and urban mobile sources characterize the NOx emissions, and the NOx emissions in nonpeak regions are primarily mobile-source emissions. ROG emissions are dominated by biogenic isoprene production in the southern United States, and they have a strong seasonal variability. CO emissions are characterized by less variability, with area and mobile sources dominating the inventory. We compare ratios of season-average nonmethane organic gases to NOx between the emission inventory and the Photochemical Assessment Monitoring Stations (PAMS) data, and these comparisons show poor correlation between the inventory and ambient ratios. [References: 21]
机译:本文描述了从区域空气质量季节性模型(SMRAQ)项目的清单准备和排放处理中获得的经验和见解。排放清单来自1990年和1995年的臭氧运输评估小组(OTAG)清单。在这里,我们概述了用于5月至9月模拟的排放处理策略,总结了OTAG库存的库存特征和更正,并描述了作为处理过程一部分采取的质量保证步骤。然后,我们提供每小时的网格排放的氮氧化物(NOx),反应性有机气体(ROG)和一氧化碳(CO)的空间图和每日总时间序列图。电力实用点源和城市移动源产生的高峰是NOx排放的特征,非高峰地区的NOx排放主要是移动源排放。 ROG排放主要由美国南部的生物异戊二烯产生,并且它们具有很强的季节性变化性。一氧化碳排放的特点是可变性较小,面积和移动源占主导地位。我们比较了排放清单和光化学评估监测站(PAMS)数据之间的季节平均非甲烷有机气体与NOx的比率,这些比较显示清单与环境比率之间的相关性较差。 [参考:21]

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