A novel approach to enhance the activity of H-form zeolite catalyst for production of hydroxymethylfurfural from cellulose

Hussein Abou-Yousef; El Barbary Hassan

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A novel approach to enhance the activity of H-form zeolite catalyst for production of hydroxymethylfurfural from cellulose

机译：增强H型沸石催化剂从纤维素生产羟甲基糠醛的活性的新方法

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Promoted H-form zeolite was demonstrated as efficient catalyst for direct conversion of cellulose into hydroxymethylfurfural (HMF) in ionic liquid. Incorporation of alkali metal chlorides with zeolite was a novel approach to enhance the catalytic activity for the H-form zeolite. The reaction conditions were optimized for the highest HMF production by changing the alkali metal chloride/H-form zeolite catalytic system. Zeolite/LiCl system was the most effective catalyst used for production of HMF and other furan compounds. A proposed mechanism explaining the role of metal chlorides in increasing the acidity of system and accelerating the hydrolysis step of cellulose was explained.

机译：促进型H型沸石被证明是在离子液体中将纤维素直接转化为羟甲基糠醛（HMF）的有效催化剂。碱金属氯化物与沸石的结合是提高H型沸石催化活性的新方法。通过改变碱金属氯化物/ H型沸石催化体系，优化了反应条件以实现最高的HMF生产。沸石/ LiCl体系是用于生产HMF和其他呋喃化合物的最有效催化剂。提出了一个解释机理的解释，该机理解释了金属氯化物在增加系统酸度和加速纤维素水解步骤中的作用。

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《Journal of industrial and engineering chemistry》 |2014年第4期|共6页
作者
Hussein Abou-Yousef; El Barbary Hassan;
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正文语种 eng
中图分类化学工业;
关键词
Microcrystalline cellulose; Ionic liquids; 5-Hydroxyfurfural; Furfural; Zeolite/metal chloride;

机译：微晶纤维素;离子液体;5-羟基糠醛;糠醛;沸石/金属氯化物;

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1. A novel approach to enhance the activity of H-form zeolite catalyst for production of hydroxymethylfurfural from cellulose [J] . Hussein Abou-Yousef, El Barbary Hassan Journal of industrial and engineering chemistry . 2014,第4期

机译：增强H型沸石催化剂从纤维素生产羟甲基糠醛的活性的新方法
2. Production of 5-hydroxymethylfurfural (HMF) from rice-straw biomass using a HSO3-ZSM-5 zeolite catalyst under assistance of sonication [J] . Hoang Phan Huy, Dat Nguyen Minh, Cuong Thai Dinh, RSC Advances . 2020,第23期

机译：在超声处理的帮助下，使用HSO3-ZSM-5沸石催化剂从水稻生物质中生产5-羟甲基糠醛（HMF）
3. Production of 5-hydroxymethylfurfural (HMF) from rice-straw biomass using a HSO3–ZSM-5 zeolite catalyst under assistance of sonication [J] . Phan Huy Hoang, Nguyen Minh Dat, Thai Dinh Cuong, RSC Advances . 2020,第23期

机译：在超声处理的帮助下，使用HSO3-ZSM-5沸石催化剂从水稻生物质中生产5-羟甲基糠醛（HMF）
4. Enhancement of the activity of CaA zeolites as deep oxidation catalysts through transition metal ion exchange [C] . E.Diaz, S.Ordonez, A.Vega, the International Zeolite Symposium . 2005

机译：通过过渡金属离子交换提高Caa沸石作为深氧化催化剂的活性
5. Fundamental Understanding of Structure-Activity Relationships for Surface Science Zeolite Model System and Zeolite Supported Metal Catalysts [D] . Akter, Nusnin. 2019

机译：对表面科学沸石模型系统和沸石负载金属催化剂结构 - 活性关系的根本理解
6. Enhancement of platelet reactivity and modulation of eicosanoid production by intact erythrocytes. A new approach to platelet activation and recruitment. [O] . M T Santos, J Valles, A J Marcus, 1991

机译：完整的红细胞增强血小板反应性并调节类花生酸的产生。血小板活化和募集的新方法。
7. Production of 5-Hydroxymethylfurfural from Direct Conversion of Cellulose Using Heteropolyacid/Nb2O5 as Catalyst [O] . Jéssica Siqueira Mancilha Nogueira, Vinícius Tomaz Santana, Paulo Vitor Henrique, 2020

机译：使用杂多酸/ Nb2O5作为催化剂从纤维素直接转化的5-羟甲基糠醛的生产

A novel approach to enhance the activity of H-form zeolite catalyst for production of hydroxymethylfurfural from cellulose

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