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Fragility measures and mode-coupling theory

机译:脆弱性测度与模式耦合理论

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摘要

The pressure-dependence of the elastic moduli of a Lennard-Jones (LJ) system is studied within mode-coupling theory (MCT). Assuming a recently proposed link between these quantities and Angell's fragility to hold, this implies that the fragility of the LJ system increases with pressure, and that this increase is mainly connected to a change in the equation of state of the liquid, and not glassy dynamics as such. (c) 2006 Elsevier B.V. All rights reserved.
机译:在模式耦合理论(MCT)中研究了Lennard-Jones(LJ)系统的弹性模量与压力的关系。假设最近提出的这些量与Angell的脆性之间存在联系,这意味着LJ系统的脆性随压力而增加,并且这种增加主要与液体状态方程的变化有关,而不与玻璃态动力学有关。因此。 (c)2006 Elsevier B.V.保留所有权利。

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