Strong and fragile liquids - A brief critique - Comment

Roland CM; Ngai KL

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Strong and fragile liquids - A brief critique - Comment

机译：强弱液体-简要评论-评论

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Recently Hedge [J. Non-Cryst. Solids 202 (1996) 164] provided a brief critique of the fragility approach to interpreting the relaxation behavior of glass-forming liquids. This classification scheme has found wide applicability, bringing out the correlation between the steepness of a liquid's fragility curve and the breadth of its relaxation spectrum. The origin of this correlation can be gleaned from the coupling model of relaxation, which relates local chemical structure and intermolecular cooperativity. Since the tatter governs both time and temperature dependencies near T-g, to a substantial extent the suggestions of Hedge [J. Non-Cryst. Solids 202 (1996) 164] concerning the origin of fragility and its correlation with non-exponentiality have been anticipated by the model.

机译：最近对冲[J.非Cryst。 [Solids 202（1996）164]对解释玻璃形成液体的松弛行为的脆性方法进行了简短的评论。该分类方案具有广泛的适用性，它揭示了液体脆性曲线的陡度与其弛豫谱的广度之间的相关性。可以从弛豫的耦合模型中收集这种相关性的起源，该模型涉及局部化学结构和分子间的协同作用。由于t杂物控制着T-g附近的时间和温度依赖性，因此在很大程度上建议使用Hedge [J.非Cryst。该模型已预见到了关于脆性起源及其与非指数相关性的固体研究（Solids 202（1996）164）。

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《Journal of Non-Crystalline Solids: A Journal Devoted to Oxide, Halide, Chalcogenide and Metallic Glasses, Amorphous Semiconductors, Non-Crystalline Films, Glass-Ceramics and Glassy Composites》 |1997年第1期|共3页
作者
Roland CM; Ngai KL;
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正文语种 eng
中图分类晶体学;
关键词
SEGMENTAL RELAXATION; EPOXIDIZED POLYISOPRENE; TEMPERATURE-DEPENDENCE; DYNAMICS; POLYMER; MOTION; BLENDS; CHAIN;

机译：段松弛;环氧聚异戊二烯;温度依赖性;动力学;聚合物;运动;共混物;链;

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1. Response to comment on "An experimental critique on the existence of fragile-to-strong transition in glass-forming liquids" [J] . Zhu W., Marple M. A. T., Lockhart M. J., Journal of Non-Crystalline Solids: A Journal Devoted to Oxide, Halide, Chalcogenide and Metallic Glasses, Amorphous Semiconductors, Non-Crystalline Films, Glass-Ceramics and Glassy Composites . 2019,第期

机译：对“玻璃形成液体脆弱转型的实验批评”评论的回应
2. Strong and fragile liquids - A brief critique - Comment [J] . Roland CM, Ngai KL Journal of Non-Crystalline Solids: A Journal Devoted to Oxide, Halide, Chalcogenide and Metallic Glasses, Amorphous Semiconductors, Non-Crystalline Films, Glass-Ceramics and Glassy Composites . 1997,第1期

机译：强弱液体-简要评论-评论
3. An experimental critique on the existence of fragile-to-strong transition in glass-forming liquids [J] . Zhu W., Marple M. A. T., Lockhart M. J., Journal of Non-Crystalline Solids: A Journal Devoted to Oxide, Halide, Chalcogenide and Metallic Glasses, Amorphous Semiconductors, Non-Crystalline Films, Glass-Ceramics and Glassy Composites . 2018,第期

机译：玻璃形成液体脆弱转型的存在实验批评
4. The fragile to strong dynamical crossover in supercooled liquids. The o-terphenyl case and its ergodicity at the dynamical arrest. [C] . Francesco Mallamace, Carmelo Corsaro, Norberto Micali, International Symposium on Slow Dynamics in Complex Systems . 2013

机译：在过冷液体中脆弱的动态交叉。 o-terphenyl案例及其动态停滞器的崇称性。
5. The orientational dynamics of fragile glass-forming liquids, an experimental test of mode-coupling theory. [D] . Brace, David Duane. 2001

机译：易碎玻璃形成液体的取向动力学，模式耦合理论的实验测试。
6. Fragile-to-strong crossover in supercooled liquids remains elusive [O] . Yael Sarah Elmatad 2011

机译：过冷液体中从脆弱到强烈的交叉仍然难以捉摸
7. An existence of universality in the dynamics of two types of glass-forming liquids - fragile liquids and strong liquids [O] . Michio Tokuyama 2020

机译：两种玻璃形成液体动力学的普遍性存在 - 脆弱的液体和强液体

Strong and fragile liquids - A brief critique - Comment

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