Supramolecular dendrimers: Convenient synthesis by programmed self-assembly and tunable thermoresponsivity

Ghosh P.S.; Hamilton A.D.

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Supramolecular dendrimers: Convenient synthesis by programmed self-assembly and tunable thermoresponsivity

机译：超分子树状大分子：通过程序化的自组装和可调的热响应性，方便合成

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We report here the noncovalent synthesis of thermosensitive dendrimers. Short oligoguanosine strands were linked to the focal point of a dendron by using "click chemistry", and quadruplex formation was used to drive the self-assembly process in the presence of metal ions. The dynamic nature of these noncovalent assemblies can be exploited to create combinatorial libraries of dendrimers as demonstrated by the co-assembly of two components. These supramolecular dendrimers showed thermoresponsive behavior that can be tuned by varying the templating cations or the number of guanines in the oligonucleotide strand.

机译：我们在这里报告了热敏树枝状聚合物的非共价合成。通过使用“点击化学”将短的寡鸟苷链连接到树突的焦点，并在金属离子存在的情况下使用四链体形成来驱动自组装过程。可以利用这些非共价组装体的动态性质来创建树枝状聚合物的组合文库，如两个组分的共同组装所证明的。这些超分子树状聚合物显示出可通过改变寡核苷酸链中的模板化阳离子或鸟嘌呤数量来调节的热响应行为。

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《Chemistry: A European journal》 |2012年第8期|共5页
作者
Ghosh P.S.; Hamilton A.D.;
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正文语种 eng
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click chemistry; self-assembly; stimuli-responsive; supramolecular dendrimers;

机译：点击化学;自组装;刺激响应;超分子树状大分子;

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1. Supramolecular dendrimers: Convenient synthesis by programmed self-assembly and tunable thermoresponsivity [J] . Ghosh P.S., Hamilton A.D. Chemistry: A European journal . 2012,第8期

机译：超分子树状大分子：通过程序化的自组装和可调的热响应性，方便合成
2. Fluorescent and thermoresponsive supramolecular systems: synthesis, self-assembly and application in percutaneous optical monitoring [J] . Chunmei Gao, Mingzhu Liu, Shaoyu Lu Journal of Materials Chemistry, B. materials for biology and medicine . 2014,第39期

机译：荧光和热响应超分子系统：合成，自组装及其在经皮光学监测中的应用
3. Janus NLO dendrimers with different peripheral functional groups: convenient synthesis and enhanced NLO performance with the aid of the Ar-Ar-F self-assembly [J] . Liu Guangchao, Liao Qiuyan, Deng Haiyu, Journal of Materials Chemistry, C. materials for optical and electronic devices . 2019,第24期

机译：Janus NLO具有不同外围官能团的树枝状大分子：借助于AR-AR-F自组装，方便的合成和增强的NLO性能
4. Synthesis of a barbell-like triblock copolymer, poly(l-lysine) dendrimer-block-poly(ethylene glycol)-block-poly(L-Lysine) dendrimer and its self-assembly with plasmid dna [C] . J.S.Choi, D.K.Joo, J.S.Park International symposium on controlled release of bioactive materials;Consumer and diversified products conference . 2000

机译：杠铃状三嵌段共聚物，聚（1-赖氨酸）树状聚合物-嵌段-聚（乙二醇）-嵌段-聚（L-赖氨酸）树状聚合物的合成及其与质粒dna的自组装
5. Development of thermoresponsive substituted poly(caprolactone)s: Synthesis, self-assembly, and drug encapsulation. [D] . Rainbolt, Elizabeth Ann. 2014

机译：热响应性取代聚己内酯的开发：合成，自组装和药物封装。
6. Supramolecular Chemistry And Self-assembly Special Feature: Dendrimers and supramolecular chemistry [O] . Jean M. J. Fréchet 2002

机译：超分子化学和自组装特征：树枝状大分子和超分子化学
7. Supramolecular dendrimers based on the self-assembly of carbazole-derived dendrons and triazine rings: liquid crystal, photophysical and electrochemical properties [O] . Castelar Susana, Barberá Joaquín, Marcos Mercedes, 2015

机译：基于咔唑衍生的树枝状分子和三嗪环自组装的超分子树枝状大分子：液晶，光物理和电化学性质
8. Programmable Self-Assembly of DNA-Dendrimer and DNA-Fullerene Nanostructures [R] . Com, R. M. 2004

机译：DNa-Dendrimer和DNa-Fullerene纳米结构的可编程自组装

Supramolecular dendrimers: Convenient synthesis by programmed self-assembly and tunable thermoresponsivity

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