Redox-selective generation of aldehydes and H_2 from alcohols under visible light

Liu Z.; Caner J.; Kudo A.; Naka H.; Saito S.

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Redox-selective generation of aldehydes and H_2 from alcohols under visible light

机译：在可见光下从醇中氧化还原选择性生成醛和H_2

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Photosynthetic dehydrogenation: Potential usefulness of visible-light-induced dehydrogenation of alcohols in organic synthesis was demonstrated, in which aldehydes and H_2 were afforded by using Ru/SrTiO_3:Rh and water (see scheme). Water was essential for the reaction. High efficiency (TON: up to 15 400 based on Rh; H2 and aldehyde evenly generated) and high selectivity were achieved.

机译：光合脱氢：证明了可见光诱导的醇在有机合成中的潜在用途，其中通过使用Ru / SrTiO_3：Rh和水提供醛和H_2（参见方案）。水对于反应是必不可少的。实现了高效率（TON：基于Rh最高可达15400; H2和醛均匀生成）和高选择性。

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《Chemistry: A European journal》 |2013年第29期|共5页
作者
Liu Z.; Caner J.; Kudo A.; Naka H.; Saito S.;
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正文语种 eng
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alcohols; aldehydes; dehydrogenation; heterogeneous photosynthesis; visible light;

机译：醇;醛;脱氢;非均相光合作用;可见光;

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专利

1. Redox-selective generation of aldehydes and H_2 from alcohols under visible light [J] . Liu Z., Caner J., Kudo A., Chemistry: A European journal . 2013,第29期

机译：在可见光下从醇中氧化还原选择性生成醛和H_2
2. Nanospheres and nanorods structured Fe_2O_3 and Fe_(2-x)Ga_xO_3 photocatalysts for visible-light mediated (λ ≥ 420 nm) H_2S decomposition and H_2 generation [J] . Esakkiappan Subramanian, Jin-Ook Baeg, Sang Mi Lee, International journal of hydrogen energy . 2009,第20期

机译：纳米球和纳米棒结构的Fe_2O_3和Fe_（2-x）Ga_xO_3光催化剂，用于可见光介导的（λ≥420 nm）H_2S分解和H_2产生
3. Highly selective, economical and efficient oxidation of alcohols to aldehydes and ketones by air and sunlight or visible light in the presence of porphyrins sensitizers [J] . Mahdi Hajimohammadi, Nasser Safari, Hamid Mofakham Green chemistry . 2011,第4期

机译：在卟啉敏化剂的存在下，通过空气和阳光或可见光将醇高度选择性，经济有效地氧化为醛和酮
4. (Invited) Controlling the Electronic Energy Structure of ZnSe-AgInSe_2 Solid Solution Nanorods for Visible-Light-Driven Photocatalytic H_2 Evolution [C] . Tsukasa Torimoto, Ko Masuoka, Tatsuya Kameyama, Meeting of the Electrochemical Society;International Meeting on Chemical Sensors . 2020

机译：（邀请）控制ZnSe-Aginse_2固溶纳米棒的电子能结构，用于可见光催化的光催化H_2进化
5. Conjugated polymers as photoredox catalysts: A new catalytic system using visible light to promote aryl aldehyde pinacol couplings [D] . Rouch, William D. 2012

机译：共轭聚合物作为光氧化还原催化剂：利用可见光促进芳基醛频哪醇偶联的新催化体系
6. Olefination of Alkyl Halides with Aldehydes by Merging Visible-Light Photoredox Catalysis and Organophosphorus Chemistry [O] . Min Jiang, Haijun Yang, Quentin Lefebvre, 2018

机译：可见光光氧化还原催化和有机磷化学合并醛与醛的烷基化
7. Photocatalytic H_2 production on trititanate nanotubes coupled with CdS and platinum nanoparticles under visible light: revisiting H_2 production and material durability [O] . Park Hyunwoong, Ou Hsin-Hung, Kim Minju, 2017

机译：在可见光下在钛酸钛纳米管上与CdS和铂纳米粒子偶联的光催化H_2产生：重新讨论H_2产生和材料耐久性

Redox-selective generation of aldehydes and H_2 from alcohols under visible light

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