Concise Multigram-Scale Synthesis of Push-Pull Tricyanofuran-Based Hemicyanines with Giant Second-Order Nonlinearity: An Alternative for Electro-optic Materials

Wissam Bentoumi; Jean-Christophe Mulatier; Pierre-Antoine Bouit; Olivier Maury; Alberto Barsella; Jean-Pierre Vola; Evelyne Chastaing; Laurent Divay; Fran?oise Soyer; Pierre Le Barny; Yann Bretonnière; Chantal Andraud

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Concise Multigram-Scale Synthesis of Push-Pull Tricyanofuran-Based Hemicyanines with Giant Second-Order Nonlinearity: An Alternative for Electro-optic Materials

机译：具有巨大二阶非线性特性的推挽式三氰呋喃三聚氰胺的精确克级合成：电光材料的另一种选择

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Highly stable and highly soluble push-pull heptamethine hemicyanines based on the tricyanofuran electron-accepting group can be prepared on a 15 g scale. The compounds display giant second-order nonlinear figure of merit, μβ of up to 31000×10~(-48) esu, and lead to a poled material with a second-order nonlinear response, r_(33) of 90 pmV~(-1) at 1.06 μm.

机译：可以以15g的规模制备基于三氰呋喃电子接受基团的高度稳定和高度可溶的推挽式七甲胺半菁。这些化合物显示出巨大的二阶非线性品质因数，μs高达31000×10〜（-48）esu，并导致极化的材料具有二阶非线性响应，r_（33）为90 pmV〜（- 1）在1.06微米。

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《Chemistry: A European journal》 |2014年第29期|共5页
作者
Wissam Bentoumi; Jean-Christophe Mulatier; Pierre-Antoine Bouit; Olivier Maury; Alberto Barsella; Jean-Pierre Vola; Evelyne Chastaing; Laurent Divay; Fran?oise Soyer; Pierre Le Barny; Yann Bretonnière; Chantal Andraud;
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正文语种 eng
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chromophores; electro-optic materials; nonlinear optics; push-pull systems;

机译：发色团;电光材料;非线性光学;推挽系统;

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1. Concise Multigram-Scale Synthesis of Push-Pull Tricyanofuran-Based Hemicyanines with Giant Second-Order Nonlinearity: An Alternative for Electro-optic Materials [J] . Wissam Bentoumi, Jean-Christophe Mulatier, Pierre-Antoine Bouit, Chemistry: A European journal . 2014,第29期

机译：具有巨大二阶非线性特性的推挽式三氰呋喃三聚氰胺的精确克级合成：电光材料的另一种选择
2. Poled Sol-Gel Materials With Heterocycle Push-Pull Chromophores that Confer Enhanced Second-Order Optical Nonlinearity [J] . Giovanna Brusatin, Alessandro Abbotto, Luca Beverina, Advanced Functional Materials . 2004,第12期

机译：具有杂环推挽生色团的极化溶胶-凝胶材料，具有增强的二阶光学非线性
3. SYNTHESIS, CHARACTERIZATION, AND SECOND-ORDER OPTICAL NONLINEARITY OF A POLYURETHANE STRUCTURE FUNCTIONALIZED WITH A HEMICYANINE DYE [J] . Moon KJ., Lee KS., Zieba J., Macromolecules . 1996,第3期

机译：半花菁染料作用的聚氨酯结构的合成，表征和二阶光学非线性
4. MOLECULAR SECOND-ORDER OPTICAL NONLINEARITY OF PUSH-PULL BISDITHIOLENE NICKEL COMPLEXES [C] . Symposium on electrical, optical, and magnetic properties of organic solid-state materials . 1998

机译：推拉式双硫醇镍络合物的分子二阶光学非线性
5. Design, synthesis and characterization of novel second-order nonlinear optical chromophores with fused-ring polyenes for application in polymeric electro-optic modulators. [D] . Todorova, Galina Krassimirova. 2000

机译：具有稠环多烯的新型二阶非线性光学生色团的设计，合成和表征，用于聚合物电光调制器。
6. Electronic Metamaterials with Tunable Second-order Optical Nonlinearities [O] . Hung-Hsi Lin, Felipe Vallini, Mu-Han Yang, -1

机译：具有可调二阶光学非线性的电子超材料
7. Push-pull systems bearing a quinoid/aromatic thieno3,2-bthiophene moiety: synthesis, ground state polarization and second-order nonlinear properties [O] . Marco A. Belén, Andreu Raquel, Franco Santiago, 2015

机译：带有醌/芳族噻吩并3,2-b噻吩部分的推挽系统：合成，基态极化和二阶非线性特性
8. Second-Order Active NLO Chromophores for DNA Based Electro-Optics Materials [R] . Andraud, C. 2010

机译：基于DNa的电光材料的二阶活性NLO生色团

Concise Multigram-Scale Synthesis of Push-Pull Tricyanofuran-Based Hemicyanines with Giant Second-Order Nonlinearity: An Alternative for Electro-optic Materials

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