Direct Assembly of 2-Oxazolidinones by Chemical Fixation of Carbon Dioxide

Teemu Niemi; Jesus E. Perea-Buceta; Israel Fernández; Sami Alakurtti; Erika Rantala; Timo Repo

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Direct Assembly of 2-Oxazolidinones by Chemical Fixation of Carbon Dioxide

机译：通过二氧化碳化学固定法直接组装2-恶唑烷酮

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The reaction of β-and γ-haloamines with carbon dioxide to give pharmaceutically relevant 2-oxazolidinones and 1,3-dioxazin-2-ones, was found to proceed efficiently in the presence of a base and in the absence of catalyst. After optimization of reaction conditions, the system was successfully expanded to a variety of haloamines, even at multigram scale. The reaction was further studied in silico by DFT calculations.

机译：发现β-和γ-卤代胺与二氧化碳的反应以产生药学上相关的2-恶唑烷酮和1，3-二恶嗪-2-酮，在碱存在下且在没有催化剂的情况下有效地进行。在优化反应条件之后，该系统成功地扩展到了多种卤代胺，即使在数克规模也是如此。通过DFT计算对反应进行了进一步的计算机研究。

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《Chemistry: A European journal》 |2014年第29期|共5页
作者
Teemu Niemi; Jesus E. Perea-Buceta; Israel Fernández; Sami Alakurtti; Erika Rantala; Timo Repo;
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正文语种 eng
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2-oxazolidones; antibiotics; carbon dioxide activation; carbon dioxide fixation; density functional calculations;

机译：2-恶唑烷酮;抗生素;二氧化碳活化;二氧化碳固定;密度泛函计算;

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1. Direct Assembly of 2-Oxazolidinones by Chemical Fixation of Carbon Dioxide [J] . Teemu Niemi, Jesus E. Perea-Buceta, Israel Fernández, Chemistry: A European journal . 2014,第29期

机译：通过二氧化碳化学固定法直接组装2-恶唑烷酮
2. Photoelectrochemical Reduction of Carbon Dioxide on Quantum-Dot-Modified Electrodes by Electric Field Directed Layer-by-Layer Assembly Methodology [J] . Guzman Diego, Isaacs Mauricio, Osorio-Roman Igor, ACS applied materials & interfaces . 2015,第36期

机译：电场定向层组装法在量子点修饰电极上光电化学还原二氧化碳
3. Direct chemical fixation of carbon dioxide to poly(GMA-co St) and the miscibility behavior of its blend with poly(MMA) [J] . D.W.Park, S.Y.Park, H.Y.Park, Preprints . 2001,第1期

机译：二氧化碳直接化学固定在聚（GMA-co St）上以及其与聚（MMA）的混溶性
4. DEVELOPMENT OF A NEW CO_2 FIXATION/UTILIZATION PROCESS (1): RECOVERY OF CALCIUM FORM STEELMAKING SLAG AND CHEMICAL FIXATION OF CARBON DIOXIDE BY CARBONATION REACTION [C] . Katsunori Yogo, Yonghong Teng, Tatsuaki Yashima, International Conference on Greenhouse Gas Control Technologies . 2005

机译：开发新的CO_2固定/利用过程（1）：通过碳化反应恢复钙塑料炼钢炉渣和二氧化碳的化学固定
5. Chemical fixation of carbon dioxide and other heterocumulenes: The development of catalysts for the reaction of epoxides and carbon dioxide/heterocumulenes . [D] . Paddock, Robert Lewis. 2004

机译：二氧化碳和其他杂聚枯烯的化学固定：环氧化物和二氧化碳/杂聚枯烯的反应催化剂的开发。
6. A possible ribosomal-directed regulatory system in Euglena gracilis. Carbon dioxide fixation [O] . R. Wolfovitch, M. Perl 1972

机译：细叶Euglena中可能存在的由核糖体控制的调节系统。二氧化碳固定
7. REL~ATIONSHIP BETWEEN LIGHT CARBON DIOXIDE FIXATION AND DARK CARBON DIOXIDE FIXATION BY MARINE ALGAE’ [O] . Ian Mowis, Clarke M. Yentsch, Charles S. Emtsch 2015

机译：海洋藻类固定二氧化碳固定与二氧化碳固定之间的关系
8. Fixation of Carbon Dioxide Coupled to Photo-Chemical Reduction of Pyridine Nucleotides by Chloroplast Preparations. [R] . Vishniac, W., Ochoa, S. 1952

机译：通过叶绿体制剂固定二氧化碳与光化学还原吡啶核苷酸相结合。

Direct Assembly of 2-Oxazolidinones by Chemical Fixation of Carbon Dioxide

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