Controlling Electron Rebound within Four-Base p-Stacks in Z-DNA by Changing the Sugar Moiety from Deoxy- to Ribonucleotide

Yuta Sannohe; Seiichiro Kizaki; Shuhei Kanesato; Ayaka Fujiwara; Yue Li; Hironobu Morinaga; Ryu Tashiro; Hiroshi Sugiyama

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Controlling Electron Rebound within Four-Base p-Stacks in Z-DNA by Changing the Sugar Moiety from Deoxy- to Ribonucleotide

机译：通过将糖部分从脱氧核苷酸更改为核糖核苷酸来控制Z-DNA的四碱基p堆栈内的电子反弹

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Charge transfer through DNA is of great interest because of the potential of DNA to be a building block for nanoelectronic sensors and devices. The photochemical reaction of 5-halouracil has been used for probing charge-transfer processes along DNA. We previously reported on unique charge transfer following photochemical reaction of 5-bromouracil within four-base p-stacks in Z-DNA. In this study, we incorporated a guanosine instead of a deoxyguanosine into Z-DNA, and found that electron transfer occurs in a different mechanism through fourbase p-stacks.

机译：通过DNA进行电荷转移非常令人感兴趣，因为DNA可能成为纳米电子传感器和设备的基础。 5-氟尿嘧啶的光化学反应已用于探测沿DNA的电荷转移过程。我们先前曾报道过Z-DNA中4个碱基的p-stack中5-溴尿嘧啶的光化学反应后的独特电荷转移。在这项研究中，我们将鸟嘌呤而不是脱氧鸟苷掺入Z-DNA中，发现通过四碱基p堆以不同的机理发生电子转移。

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《Chemistry: A European journal》 |2014年第5期|共3页
作者
Yuta Sannohe; Seiichiro Kizaki; Shuhei Kanesato; Ayaka Fujiwara; Yue Li; Hironobu Morinaga; Ryu Tashiro; Hiroshi Sugiyama;
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正文语种 eng
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关键词
5-bromouracil; excess electron transfer; four-base p-stacks; z-dna;

机译：5-溴尿嘧啶;过量电子转移;四基p堆;z-dna;

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1. Controlling Electron Rebound within Four-Base p-Stacks in Z-DNA by Changing the Sugar Moiety from Deoxy- to Ribonucleotide [J] . Yuta Sannohe, Seiichiro Kizaki, Shuhei Kanesato, Chemistry: A European journal . 2014,第5期

机译：通过将糖部分从脱氧核苷酸更改为核糖核苷酸来控制Z-DNA的四碱基p堆栈内的电子反弹
2. Deoxygenative [1,2]-Hydride Shift Rearrangements in Nucleosidse and Sugar Chemistry: Analogy with the [1,2]-Electron Shift in the Deoxygenation of Ribonucleotides by Ribonucleotide Reductases [J] . Morris J. Robins, Ireneusz Nowak, Stanislaw F. Wnuk, The Journal of Organic Chemistry . 2007,第22期

机译：核苷酸和糖化学中的脱氧性[1,2]-氢化物移位重排：与核糖核苷酸还原酶的核糖核苷酸脱氧中的[1,2]-电子移位相似
3. Multiple Controls Regulate the Expression of mobE, an HNH Homing Endonuclease Gene Embedded within a Ribonucleotide Reductase Gene of Phage Aeh1 [J] . Ewan A. Gibb, David R. Edgell Journal of bacteriology . 2007,第13期

机译：多个控件调节mobE的表达，mobE是一种嵌入噬菌体Aeh1的核糖核苷酸还原酶基因中的HNH归巢核酸内切酶基因。
4. On decentralized control of small loads and energy rebound within primary frequency control [C] . Arnaud Latiers, Francois Glineur, Emmanuel De Jaeger, Power Systems Computation Conference . 2016

机译：一次频率控制内的小负荷分散控制和能量回弹
5. Protein structural changes and tyrosyl radical-mediated electron transfer reactions in ribonucleotide reductase and model compounds [D] . Offenbacher, Adam R. 2010

机译：核糖核苷酸还原酶和模型化合物中的蛋白质结构变化和酪氨酰自由基介导的电子转移反应
6. Formation of Z-DNA in negatively supercoiled plasmids is sensitive to small changes in salt concentration within the physiological range. [O] . F Azorin, A Nordheim, A Rich 1983

机译：负超螺旋质粒中Z-DNA的形成对生理范围内盐浓度的微小变化敏感。
7. Deoxygenative 1,2-Hydride Shift Rearrangements in Nucleoside and Sugar Chemistry: Analogy with the 1,2-Electron Shift in the Deoxygenation of Ribonucleotides by Ribonucleotide Reductases [O] . -1

机译：核苷和糖化学的脱氧1,2-rydride换档重排：通过核糖核苷酸还原酶对核糖核苷酸的脱氧中的1,2 - 电子转移进行类比

Controlling Electron Rebound within Four-Base p-Stacks in Z-DNA by Changing the Sugar Moiety from Deoxy- to Ribonucleotide

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