Synthesis, Electronic Properties and WOLED Devices of Planar Phosphorus-Containing Polycyclic Aromatic Hydrocarbons

Riobe Francois; Szucs Rozsa; Bouit Pierre-Antoine; Tondelier Denis; Geffroy Bernard; Aparicio Fatima; Buendia Julia; Sanchez Luis; Reau Regis; Nyulaszi Laszlo; Hissler Muriel

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Synthesis, Electronic Properties and WOLED Devices of Planar Phosphorus-Containing Polycyclic Aromatic Hydrocarbons

机译：平面含磷多环芳烃的合成，电子性质及WOLED器件

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We describe the synthesis and the physical properties of polyaromatic hydrocarbons (PAHs) containing a phosphorus atom at the edge. In particular, the impact of the successive addition of aromatic rings on the electronic properties was investigated by experimental (UV/Vis absorption, fluorescence, cyclic voltammetry) and theoretical studies (DFT). The physical properties recorded in solution and in the solid state showed that the P-containing PAHs exhibit properties expected for an emitter in white organic light-emitting diodes (WOLEDs).

机译：我们描述了在边缘含有磷原子的聚芳烃（PAHs）的合成和物理性质。特别地，通过实验（UV / Vis吸收，荧光，循环伏安法）和理论研究（DFT）研究了连续添加芳环对电子性能的影响。在溶液和固态下记录的物理性质表明，含P的PAH表现出白色有机发光二极管（WOLED）中的发射极所期望的性质。

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来源
《Chemistry: A European journal》 |2015年第17期|共10页
作者
Riobe Francois; Szucs Rozsa; Bouit Pierre-Antoine; Tondelier Denis; Geffroy Bernard; Aparicio Fatima; Buendia Julia; Sanchez Luis; Reau Regis; Nyulaszi Laszlo; Hissler Muriel;
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正文语种 eng
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aromaticity; electronic structure; energy conversion; phosphorus heterocycles; pi interactions;

机译：芳香性;电子结构;能量转换;磷杂环;π相互作用;

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1. Synthesis, Electronic Properties and WOLED Devices of Planar Phosphorus-Containing Polycyclic Aromatic Hydrocarbons [J] . Riobe Francois, Szucs Rozsa, Bouit Pierre-Antoine, Chemistry: A European journal . 2015,第17期

机译：平面含磷多环芳烃的合成，电子性质及WOLED器件
2. The Delocalization Index as an Electronic Aromaticity Criterion: Application to a Series of Planar Polycyclic Aromatic Hydrocarbons [J] . Jordi Poater, Xavier Fradera, Miquel Duran, Chemistry: A European journal . 2003,第2期

机译：作为电子芳香性标准的离域指数：在一系列平面多环芳香烃中的应用
3. Quantum Mechanical-Based Quantitative Structure–Property Relationships for Electronic Properties of Two Large Classes of Organic Semiconductor Materials: Polycyclic Aromatic Hydrocarbons and Thienoacenes [J] . Lam H. Nguyen, Tuan H. Nguyen, Thanh N. Truong ACS Omega . 2019,第4期

机译：Quantum基于机械的定量结构 - 性能与电子性质的两种大类有机半导体材料的性能关系：多环芳烃和噻吩苯乙烯
4. Polycyclic aromatic hydrocarbons (PAHs) have much received attention as one of thefundamental components of organic devices.1 Although PAHs are usually composed ofhexagons (benzenoid systems),embedding odd-membered rings such as pentagons orheptagons (non-benzenoid systems) into the molecular core is a promising methodology tomodify their electronic properties,such as aromaticity,redox ability and/or spin state [C] . Koki Horii, Akihito Konishi, MakotoYasuda 日本化学会春季年会 . 2020

机译：多环芳烃（PAHS）作为有机器件的金融组件之一，多环芳烃（PAHS）有很多人受到关注.1虽然PAHS通常由过爆（苯甲酸系统）组成，但嵌入奇数元环，例如Pentagons Orheptagons（非苯骨系统）进入分子核心是一个有希望的方法，可以清理它们的电子性质，例如芳香性，氧化还原能力和/或旋转状态
5. Fluoroalkyl and Fluoroaryl Fullerenes, Polycyclic Aromatic Hydrocarbons, and Copper(I) Complexes: Synthesis, Structure, Electrochemical, Photophysical, and Device Properties [D] . Reeves, Brian J. 2020

机译：氟代烷基和氟芳基富勒烯，多环芳烃和铜（I）配合物：合成，结构，电化学，光药和装置性能
6. Quantum Mechanical-Based Quantitative Structure–PropertyRelationships for Electronic Properties of Two Large Classes of OrganicSemiconductor Materials: Polycyclic Aromatic Hydrocarbons and Thienoacenes [O] . Lam H. Nguyen, Tuan H. Nguyen, Thanh N. Truong, 2019

机译：基于量子力学的定量结构-性质两大类有机物的电子性质关系半导体材料：多环芳烃和硫杂环丁烷
7. Synthesis, Electronic Properties and WOLED Devices of Planar Phosphorus-Containing Polycyclic Aromatic Hydrocarbons [O] . Riobé François, Szűcs Rózsa, Bouit Pierre-Antoine, 2015

机译：平面含磷多环芳烃的合成，电子性质及WOLED器件
8. Investigation of the Distribution of Organochlorine and Polycyclic Aromatic211 Hydrocarbon Compounds in the Lower Columbia River Using Semipermeable Membrane 211 Devices [R] . McCarthy, K. A., Gale, R. W. 1999

机译：利用半透膜211装置研究哥伦比亚河下游有机氯和多环芳烃211烃类化合物的分布

Synthesis, Electronic Properties and WOLED Devices of Planar Phosphorus-Containing Polycyclic Aromatic Hydrocarbons

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