Selective ionization via different electronic pathways by optimal control demonstrated for (NaK)-Na-23-K-39/(NaK)-Na-23-K-41

Lindinger A; Vetter F; Lupulescu C; Plewicki M; Weber SM; Merli A; Woste L

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Selective ionization via different electronic pathways by optimal control demonstrated for (NaK)-Na-23-K-39/(NaK)-Na-23-K-41

机译：通过（NaK）-Na-23-K-39 /（NaK）-Na-23-K-41的最佳控制通过不同电子途径进行选择性电离

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Selective optimization of different isotopomers in an ionization process with shaped fs-laser pulses is presented for (NaK)-Na-23-K-39/(NaK)-Na-23-K-41. By employing evolution strategies in a closed feedback loop a considerably high enhancement by a total factor of about 25 of one isotope compared to the other and reversed is measured. Surprisingly, vibrational levels of differing electronic states are utilized for the different isotopomer selections. Our approach generally allows to influence vibrational wave functions by coherent interaction with the corresponding spectral pulse components on the fs-time scale. (C) 2004 Elsevier B.V. All rights reserved.

机译：针对（NaK）-Na-23-K-39 /（NaK）-Na-23-K-41提出了具有定型fs-激光脉冲的电离过程中不同同位素的选择性优化。通过在封闭的反馈回路中采用演化策略，可以测量一种同位素与另一种同位素的总和提高了约25倍，并且得到了相当大的提高。令人惊讶地，不同电子态的振动水平被用于不同的同位素选择。我们的方法通常允许通过与fs时间尺度上的相应频谱脉冲分量的相干相互作用来影响振动波函数。（C）2004 Elsevier B.V.保留所有权利。

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来源
《Chemical Physics Letters》 |2004年第3期|共5页
作者
Lindinger A; Vetter F; Lupulescu C; Plewicki M; Weber SM; Merli A; Woste L;
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正文语种 eng
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关键词
FEMTOSECOND LASER-PULSES; A(1)SIGMA(+) STATE; ISOTOPE-SEPARATION; NAK; OPTIMIZATION; DISSOCIATION; CLUSTERS; DYNAMICS;

机译：飞秒激光;A（1）SIGMA（+）状态;同位素分离;NAK;优化;解离;群体;动态;

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专利

1. Selective ionization via different electronic pathways by optimal control demonstrated for (NaK)-Na-23-K-39/(NaK)-Na-23-K-41 [J] . Lindinger A, Vetter F, Lupulescu C, Chemical Physics Letters . 2004,第1a3期

机译：通过（NaK）-Na-23-K-39 /（NaK）-Na-23-K-41的最佳控制通过不同电子途径进行选择性电离
2. Optimized isotope-selective ionization of (NaK)-Na-23-K-39 and (NaK)-Na-23-K-41 by applying evolutionary strategies [J] . Vetter F, Plewicki M, Lindinger A, Physical chemistry chemical physics: PCCP . 2005,第6期

机译：通过应用进化策略优化（NaK）-Na-23-K-39和（NaK）-Na-23-K-41的同位素选择性电离
3. Parametric polarization pulse shaping demonstrated for optimal control of NaK [J] . Weber SM, Plewicki M, Weise F, The Journal of Chemical Physics . 2008,第17期

机译：演示了参数极化脉冲整形可实现NaK的最佳控制
4. Controlling the dynamical pathways in the ionization processes of NaK dimers [C] . Albrecht Lindinger, Stefan M. Weber, Andrea Merli, International Conference on Femtochemistry . 2006

机译：控制NAK二聚体电离过程中的动态途径
5. Ion Selectivity and Allostery in the NaK Channel. [D] . Brettmann, Joshua Blain. 2015

机译：NaK通道中的离子选择性和变构作用。
6. Intracellular Na+ Controls Cell Surface Expression of NaK-ATPase via a cAMP-independent PKA Pathway in Mammalian Kidney Collecting Duct Cells [O] . Manlio Vinciguerra, Georges Deschênes, Udo Hasler, 2003

机译：细胞内Na +控制细胞的表面表达 NaK-ATPase通过哺乳动物肾脏收集中不依赖cAMP的PKA途径导管细胞
7. Hydration valve controlled non-selective conduction of Na+ and K+ in the NaK channel [O] . Shen Rong, Guo Wanlin, Zhong Wenyu 2010

机译：水化阀控制NaK通道中Na +和K +的非选择性传导

Selective ionization via different electronic pathways by optimal control demonstrated for (NaK)-Na-23-K-39/(NaK)-Na-23-K-41

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