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Two stages of Kondo effect and competition between RKKY and Kondo in Gd-based intermetallic compound

机译:G基金属间化合物中近藤效应的两个阶段以及近畿近藤与KKD之间的竞争

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The magnetic behavior of Gd-based intermetallic compound (Gd2Al(1-x)Aux) in the form of the powder and needle, is investigated. All the samples are an orthorhombic crystal structure. Only the compound with x = 0.4 shows the Kondo effect (other compounds have a normal behavior). Although, for the compound in the form of powder, with x = 0.4, the susceptibility measurement X(T) shows two different stages. Moreover for (T > T-K2) a fall of the value of chi(T) is observable, which indicates a weak presence of ferromagnetic phase. About the two stages of Kondo effect, we observe at the first (T-K1) an increase of X(T) and in the second stage (T-K2) a new remarkable decrease of chi(T), (T-K1 > T-K2). For the sample in the form of needles, the first stage is observable only under high magnetic field. This first stage could be corresponds to a narrow resonance between Kondo cloud and itinerant electron. The second stage, which is remarkably visible for the sample in the form of the powder, can be attribute to a complete polarization of Kondo cloud. Observation of these two Kondo stages could be due to the weak presence of RKKY contribution. (c) 2006 Published by Elsevier B.V.
机译:研究了粉末和针状Gd基金属间化合物(Gd2Al(1-x)Aux)的磁行为。所有样品均为正交晶体结构。只有x = 0.4的化合物显示近藤效应(其他化合物具有正常行为)。尽管对于粉末形式的化合物,当x = 0.4时,磁化率测量值X(T)显示出两个不同的阶段。此外,对于(T> T-K2),可观察到chi(T)值下降,这表明铁磁相的存在很弱。关于近藤效应的两个阶段,我们在第一阶段(T-K1)观察到X(T)的增加,而在第二阶段(T-K2)观察到chi(T)的新的显着下降,(T-K1> T-K2)。对于针状样品,只有在强磁场下才能观察到第一阶段。该第一阶段可能对应于近藤云与流动电子之间的窄共振。第二阶段对粉末形式的样品来说非常明显,这可以归因于近藤云的完全极化。观察这两个近藤阶段可能是由于RKKY贡献的存在不足。 (c)2006年由Elsevier B.V.

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