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Laser-induced reconstruction of Ag clusters in helium droplets

机译:激光诱导氦滴中银团簇的重建

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Silver clusters were assembled in helium droplets of different sizes ranging from 10(5) to 10(10) atoms. The absorption of the clusters was studied upon laser irradiation at 355 nm and 532 nm, which is close to the plasmon resonance maximum in spherical Ag clusters and in the range of the absorption of the complex, branched Ag clusters, respectively. The absorption of the pulsed (7 ns) radiation at 532 nm shows some pronounced saturation effects, absent upon the continuous irradiation. This phenomenon has been discussed in terms of the melting of the complex Ag clusters at high laser fluence, resulting in a loss of the 532 nm absorption. Estimates of the heat transfer also indicate that a bubble may be formed around the hot cluster at high fluences, which may result in ejection of the cluster from the droplet, or disintegration of the droplet entirely. Published by AIP Publishing.
机译:银簇被组装成10至5至10至10个原子大小的不同氦气滴。在355 nm和532 nm的激光辐照下研究了团簇的吸收,这接近于球形Ag团簇中的等离激元共振最大值,并且分别接近于复杂的,分支的Ag团簇的吸收范围。 532 nm的脉冲(7 ns)辐射的吸收显示出一些明显的饱和效应,而连续辐射则不存在。已经就高激光通量下复杂银团簇的熔化讨论了这一现象,导致532 nm吸收的损失。传热的估计值还表明,在热簇周围可能会以高通量形成气泡,这可能导致簇从液滴中喷出或完全崩解。由AIP Publishing发布。

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