LiClO_4 Electrolyte Solvate Structures

Wesley A. Henderson; Neil R. Brooks; William W. Brennessel; Victor G. Young Jr.

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LiClO_4 Electrolyte Solvate Structures

机译：LiClO_4电解质溶剂化结构

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Two crystalline phases, (monoglyme)_2:LiClO_4 and (diglyme)_2:LiClO_4, have been isolated and characterized. The former consists of contact ion pairs in which the anions have bidentate coordination to the Li~+ cations, while the latter consists of fully solvated Li~+ cations in which the cations and anions do not directly interact. The two structures are useful as models for solvate structures in concentrated electrolyte mixtures. In particular, the phase behavior and solvate structures of solvent-salt mixtures are informative when coupled with vibrational spectroscopic analysis of ionic association behavior in solutions.

机译：（monoglyme）_2：LiClO_4和（diglyme）_2：LiClO_4这两个结晶相已被分离和表征。前者由接触离子对组成，其中阴离子与Li〜+阳离子具有双齿配位，而后者由完全溶剂化的Li〜+阳离子组成，其中阳离子和阴离子不直接相互作用。这两种结构可用作浓电解质混合物中溶剂化物结构的模型。尤其是，当与溶液中离子缔合行为的振动光谱分析结合使用时，溶剂盐混合物的相行为和溶剂化物结构将非常有用。

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《The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory》 |2004年第1期|共5页
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Wesley A. Henderson; Neil R. Brooks; William W. Brennessel; Victor G. Young Jr.;
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1. LiClO_4 Electrolyte Solvate Structures [J] . Wesley A. Henderson, Neil R. Brooks, William W. Brennessel, The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory . 2004,第1期

机译：LiClO_4电解质溶剂化结构
2. Chelate Effects in Glyme/Lithium Bis(trifluoromethanesulfonyl)amide Solvate Ionic Liquids, Part 2: Importance of Solvate-Structure Stability for Electrolytes of Lithium Batteries [J] . Ce Zhang, Azusa Yamazaki, Junichi Murai The journal of physical chemistry, C. Nanomaterials and interfaces . 2014,第31期

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3. Chelate Effects in Glyme/Lithium Bis(trifluoromethanesulfonyl)amide Solvate Ionic Liquids, Part 2: Importance of Solvate-Structure Stability for Electrolytes of Lithium Batteries [J] . Ce Zhang, Azusa Yamazaki, Junichi Murai The journal of physical chemistry, C. Nanomaterials and interfaces . 2014,第31期

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4. LiBETI Solvate Structures and Ionic Association Interactions in Electrolytes [C] . Wesley A.Henderson, William H.Smyrl, Neil R.Brooks, The Meeting of the Electrochemical Society . 2003

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LiClO_4 Electrolyte Solvate Structures

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