Chemical Reaction Studies in CH_4/Ar and CH_4/N_2 Gas Mixtures of a Dielectric Barrier Discharge

Abhijit Majumdar; Jurgen F.Behnke; Rainer Hippler; Konstantin Matyash; Ralf Schneider

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Chemical Reaction Studies in CH_4/Ar and CH_4/N_2 Gas Mixtures of a Dielectric Barrier Discharge

机译：介质阻挡放电的CH_4 / Ar和CH_4 / N_2气体混合物中的化学反应研究

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Chemical reactions in a dielectric barrier discharge at medium pressure of 250-300 mbar have been studied in CH_4/Ar and CH_4/N_2 gas mixtures by means of mass spectrometry.The main reaction scheme is production of H_2 by fragmentation of CH_4,but also production of higher order hydrocarbon molecules such as C_nH_m with n up to 9 including formation of different functional CN groups is observed.Formation of C_2H_2,C_2H_4,and C_2H_6 molecules has been investigated in some detail.Significant differences are noted in comparison to a theoretical estimate.

机译：通过质谱研究了CH_4 / Ar和CH_4 / N_2混合气体在250-300 mbar中压下介质阻挡放电中的化学反应。主要反应方案是通过CH_4的裂解生成H_2，但也有生产观察到n个多达9个的高阶碳氢化合物分子（例如C_nH_m）包括不同官能团的CN形成。已对C_2H_2，C_2H_4和C_2H_6分子的形成进行了详细研究，与理论估计值相比存在明显差异。

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《The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory》 |2005年第41期|共7页
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Abhijit Majumdar; Jurgen F.Behnke; Rainer Hippler; Konstantin Matyash; Ralf Schneider;
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1. Chemical Reaction Studies in CH_4/Ar and CH_4/N_2 Gas Mixtures of a Dielectric Barrier Discharge [J] . Abhijit Majumdar, Jurgen F.Behnke, Rainer Hippler, The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory . 2005,第41期

机译：介质阻挡放电的CH_4 / Ar和CH_4 / N_2气体混合物中的化学反应研究
2. Chemical Reaction Studies in CH_4/Ar and CH_4/N_2 Gas Mixtures of a Dielectric Barrier Discharge [J] . Abhijit Majumdar, Jurgen F.Behnke, Rainer Hippler, The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory . 2005,第41期

机译：介质阻挡放电的CH_4 / Ar和CH_4 / N_2气体混合物中的化学反应研究
3. Comparative Plasma Chemical Reaction Studies of CH_4/Ar and C_2H_m/Ar (m = 2, 4, 6) Gas Mixtures in a Dielectric Barrier Discharge [J] . H. C. Thejaswini, S. Peglow, U. Martens, Contributions to Plasma Physics . 2014,第8期

机译：介质阻挡放电中CH_4 / Ar和C_2H_m / Ar（m = 2，4，6）气体混合物的等离子体化学反应比较研究
4. Ignition of CH_4:O_2:Ar and n-C_4H_(10):O_2:Ar(N_2) mixtures with initial temperatures between 650-950 K by a surface pulsed discharge [C] . S. A. Stepanyan, M. A. Boumehdi, G. Vanhove, AIAA SciTech forum;Aerospace sciences meeting . 2014

机译：通过表面脉冲放电点燃初始温度在650-950 K之间的CH_4：O_2：Ar和n-C_4H_（10）：O_2：Ar（N_2）混合物
5. CARS thermometry studies of plasma assisted combustion in ethylene-air and hydrogen-air mixtures and of a dielectric barrier discharge actuator. [D] . Zuzeek, Yvette Marie. 2010

机译：对乙烯-空气和氢气-空气混合物中的等离子体辅助燃烧以及介电势垒放电执行器进行CARS测温研究。
6. Fast gas heating in N2/O2 mixtures under nanosecond surface dielectric barrier discharge: the effects of gas pressure and composition [O] . M. M Nudnova, S. V Kindysheva, N. L Aleksandrov, -1

机译：纳秒表面介电势垒放电下N2 / O2混合物中的快速气体加热：气体压力和组成的影响
7. An investigation of dielectric barrier discharge in Ar and Ar/NH3mixture using cross-correlation spectroscopy [O] . P Kloc, H-E Wagner, D Trunec, 2010

机译：使用互相关光谱法在Ar和Ar / NH3Mixture中的介质阻挡放电研究
8. Diffuse Dielectric Barrier Discharges in Nitrogen-Containing Gas Mixture. [R] . Brandenburg, R., Wagner, H., Michel, P., 2003

机译：含氮气体混合物中的扩散介质阻挡放电。

Chemical Reaction Studies in CH_4/Ar and CH_4/N_2 Gas Mixtures of a Dielectric Barrier Discharge

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