Reply to the Comment on 'Are Vibrationally Excited Molecules a Clue for the O_3 Deficit Problem and HO_x Dilemma in the Middle Atmosphere?'

A.J.C.Varandas

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Reply to the Comment on 'Are Vibrationally Excited Molecules a Clue for the O_3 Deficit Problem and HO_x Dilemma in the Middle Atmosphere?'

机译：对“中部大气O_3赤字问题和HO_x困境是否有振动激发分子的线索？”的评论答复

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Concerning the Comment by Smith and Copeland (SC) on my recent paper,I note the following.First,I address their remark that I have taken the input H-atom concentrations from Figure 15.2 of the textbook by Steinfeld,Francisco,and Hase.This is an excellent textbook,and I trusted that any quantitative differences from other measurements should not be of the utmost concern.In fact,despite the commented two-orders-of-magnitude difference with other measured H amounts,the general conclusions then reported will be shown to remain largely unaffected.Moreover,the SC point of view may not be shared by other atmospheric researchers.For example,Takahashi et al.report H amounts derived from simultaneous measurements of the vertical profiles of upper atmospheric airglow emissions and atmospheric sodium that vary from 10~9 cm~(-3) at 85 km to 10~8 cm~(-3) at 100 km.Besides remarking on satellite data taken in the equatorial region that show both [H] and [O_3] to have strong semiannual variations,they emphasize that their

机译：关于史密斯和科普兰（SC）在我最近的论文中的评论，请注意以下几点：首先，我解决他们的评论，即我从Steinfeld，Francisco和Hase的教科书图15.2中选取了输入的H原子浓度。这是一本非常好的教科书，我相信与其他测量值之间的任何数量差异都不应引起最大的关注。事实上，尽管与其他测得的H量之间存在两个数量级的差异，但随后得出的一般结论将而且，其他大气研究人员可能不会共享SC的观点。例如，Takahashi等人报告了同时测量高层大气气辉发射和大气钠的垂直剖面而得出的H量，从85 km时的10〜9 cm〜（-3）到100 km时的10〜8 cm〜（-3）。此外，在赤道区域拍摄的卫星数据也表明[H]和[O_3]都具有半年度变化很大强调他们

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《The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory》 |2005年第11期|共3页
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1. Reply to the Comment on "Are Vibrationally Excited Molecules a Clue for the O_3 Deficit Problem and HO_x Dilemma in the Middle Atmosphere?" [J] . A.J.C.Varandas The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory . 2005,第11期

机译：对“中部大气O_3赤字问题和HO_x困境是否有振动激发分子的线索？”的评论答复
2. Comment on "Are Vibrationally Excited Molecules a Clue for the O_3 Deficit Problem and HO_x Dilemma in the Middle Atmosphere?" [J] . Gregory P.Smith, Richard A.Copeland The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory . 2005,第11期

机译：评论“中部大气O_3赤字问题和HO_x难题是否为振动激发分子的线索？”
3. Are Vibrationally Excited Molecules a Clue for the "O_3 Deficit Problem" and "HO_x Dilemma" in the Middle Atmosphere? [J] . A. J. C. Varandas The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory . 2004,第5期

机译：振动激发分子是中层大气“ O_3缺陷问题”和“ HO_x难题”的线索吗？
4. Collisional Energy Transfer of Highly Vibrationally Excited Polyatomic Molecules. Effect of Excited Molecule Complexity [C] . Zalesskaya, G.A., Yakovlev, . 1996

机译：高振动激发多原子分子的碰撞能量转移。激发分子复杂性的影响
5. Collision-induced vibration relaxation of highly vibrationally excited molecules. [D] . Zhang, Min. 2007

机译：碰撞引起的高振动激发分子的振动弛豫。
6. Chemical Dynamics Special Feature: Chemical dynamics of vibrationally excited molecules: Controlling reactions in gases and on surfaces [O] . F. Fleming Crim 2008

机译：化学动力学特性：振动激发分子的化学动力学：控制气体和表面上的反应
7. Are Vibrationally Excited Molecules a Clue for the “O3 Deficit Problem” and “HOx Dilemma” in the Middle Atmosphere? [O] . Varandas A. J. C. 2004

机译：振动激发分子是中层大气“ O3缺陷问题”和“ HOx困境”的线索吗？
8. Average Vibrational Energy Transfer During a Single Collision of Excited Molecules with Heat Bath Molecules [R] . Oref, I., Rabinovitch, B. S. 1983

机译：激发分子与热浴分子单次碰撞时的平均振动能量转移

Reply to the Comment on 'Are Vibrationally Excited Molecules a Clue for the O_3 Deficit Problem and HO_x Dilemma in the Middle Atmosphere?'

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