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首页> 外文期刊>The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory >Photodissociation of H_2~+ upon Exposure to an Intense Pulsed Photonic Fock State
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Photodissociation of H_2~+ upon Exposure to an Intense Pulsed Photonic Fock State

机译：H_2〜+在强脉冲光子Fock状态下的光解离

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摘要

Producing and controlling nonclassical light states are now the subject of intense experimental efforts. In this paper we consider the interaction of such a light state with a small molecule. Specifically, we develop the theory and apply it numerically to calculate in detail how a short pulse of nonclassical light, such as the high intensity Fock state, induces photodissociation in H_2~+. We compare the kinetic energy distributions and photodissociation yields with the analogous results of quasi-classical light, namely a coherent state. We find that Fock-state light decreases the overall probability of dissociation for low vibrational states of H2+ as well as the location of peaks and line shapes in the kinetic energy distribution of the nuclei.
机译：如今，产生和控制非经典光态已成为实验的重点。在本文中，我们考虑了这种轻状态与小分子的相互作用。具体来说，我们发展了该理论并将其数值应用来详细计算非经典光的短脉冲（例如高强度Fock状态）如何引起H_2〜+中的光解离。我们将动能分布和光解离产率与准经典光（即相干态）的相似结果进行比较。我们发现，Fock态光降低了H2 +的低振动态的整体解离概率，以及原子核动能分布中峰和线形的位置。

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