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Mechanism for Optical Enhancement and Suppression of Fluorescence

机译:光学增强和抑制荧光的机理

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摘要

When fluorescence from electronically excited states follows the absorption of radiation, the emission spectrum is often a key to identification of the excited species. It now emerges that passing off-resonant laser light through such an electronically excited system may enhance or suppress the fluorescent emission. This report establishes the mechanism and theory for this optical control of spontaneous fluorescence, derived by quantum electrodynamical analysis. Experimental techniques to detect the enhanced signal are also proposed.
机译:当来自电子激发态的荧光跟随辐射的吸收时,发射光谱通常是识别激发物种的关键。现在显示出,使共振后的激光通过这种电子激发系统可以增强或抑制荧光发射。本报告建立了通过量子电动力学分析得出的自发荧光光学控制的机理和理论。还提出了检测增强信号的实验技术。

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