Inclined N-2 desorption in a steady-state N2O+COreaction on Pd(110)

Ma YS; Kobal I; Matsushima T

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Inclined N-2 desorption in a steady-state N2O+COreaction on Pd(110)

机译：在Pd（110）上的稳态N2O + CO反应中倾斜的N-2解吸

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The angular and velocity distributions of desorbing products were analyzed in the course of a catalyzed N2O + CO reaction oil Pd(110). The reaction proceeded steadily above 450 K, and the N-2 desorption merely collimated sharply along 45degrees off the surface normal toward the [001] direction. It is proposed that this peculiar N-2 desorption is induced by the decomposition of adsorbed N2O oriented along the [001] direction. On the basis of the observation of similar inclined N-2 desorption in both NO + CO and N2O + CO reactions, the N-2 formation via the intermediate N2O(a) dissociation was confirmed in catalytic NO reduction.

机译：在催化的N2O + CO反应油Pd（110）的过程中分析了解吸产物的角度和速度分布。反应在450 K以上稳定地进行，并且N-2解吸仅沿垂直于[001]方向的法线沿45度急剧准直。提出这种特殊的N-2解吸是由沿[001]方向取向的被吸附N2O分解引起的。基于观察到在NO + CO和N2O + CO反应中类似的倾斜N-2解吸，在催化NO还原过程中证实了通过中间N2O（a）分解形成N-2。

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《The journal of physical chemistry, B. Condensed matter, materials, surfaces, interfaces & biophysical》 |2005年第2期|共3页
作者
Ma YS; Kobal I; Matsushima T;
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正文语种 eng
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关键词
PLUS CO REACTION; REMOVAL PATHWAYS; NO; ADSORPTION; SURFACE; DECOMPOSITION; NITROGEN; MODEL;

机译：PLUS CO反应;去除途径;否;吸附;表面;分解;氮;模型;

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1. Inclined N-2 desorption in a steady-state N2O+COreaction on Pd(110) [J] . Ma YS, Kobal I, Matsushima T The journal of physical chemistry, B. Condensed matter, materials, surfaces, interfaces & biophysical . 2005,第2期

机译：在Pd（110）上的稳态N2O + CO反应中倾斜的N-2解吸
2. Inclined N-2 desorption in a steady-state NO plus CO reaction on Pt(100) [J] . Horino H, Matsushima T The journal of physical chemistry, B. Condensed matter, materials, surfaces, interfaces & biophysical . 2005,第2期

机译：在Pt（100）的稳态NO加CO反应中倾斜的N-2解吸
3. Inclined N-2 desorption in N2O decomposition on Rh(110) [J] . Matsushima T, Imamura K, Horino H, Applied Surface Science . 2005,第1a4期

机译：Rh（110）上N2O分解中的倾斜N-2解吸
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5. Adatom diffusion and interactions: Pd on W(110). [D] . Koh, Seong Jin. 1998

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Inclined N-2 desorption in a steady-state N2O+COreaction on Pd(110)

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