Fixation of atmospheric carbon dioxide by ruthenium complexes bearing an NHC-based pincer ligand: formation of a methylcarbonato complex and its methylation

Arikawa Yasuhiro; Nakamura Takuo; Ogushi Shinji; Eguchi Kazushige; Umakoshi Keisuke

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Fixation of atmospheric carbon dioxide by ruthenium complexes bearing an NHC-based pincer ligand: formation of a methylcarbonato complex and its methylation

机译：带有基于NHC的钳形配体的钌配合物固定大气中的二氧化碳：甲基碳酸酯配合物的形成及其甲基化

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A methylcarbonato ruthenium complex was prepared by capture of CO2 from air using the (CNC)(bpy)Ru scaffold. The methylcarbonato complex was relatively inert to decarboxylation. Treatments with methylating reagents released dimethylcarbonate.

机译：通过使用（CNC）（bpy）Ru支架从空气中捕获CO2来制备甲基碳酸钌复合物。甲基碳酸酯络合物对脱羧相对惰性。用甲基化试剂处理释放出碳酸二甲酯。

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《Dalton transactions: An international journal of inorganic chemistry》 |2015年第12期|共3页
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Arikawa Yasuhiro; Nakamura Takuo; Ogushi Shinji; Eguchi Kazushige; Umakoshi Keisuke;
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1. Fixation of atmospheric carbon dioxide by ruthenium complexes bearing an NHC-based pincer ligand: formation of a methylcarbonato complex and its methylation [J] . Arikawa Yasuhiro, Nakamura Takuo, Ogushi Shinji, Dalton transactions: An international journal of inorganic chemistry . 2015,第12期

机译：带有基于NHC的钳形配体的钌配合物固定大气中的二氧化碳：甲基碳酸酯配合物的形成及其甲基化
2. A Series of Cu(II) Complexes Based on Different Bis(imidazole) Ligands and Organic Acids: Formation of Water Clusters and Fixation of Atmospheric Carbon Dioxide [J] . Yang J, Ma JF, Liu YY, Crystal growth & design . 2008,第12期

机译：基于不同双（咪唑）配体和有机酸的一系列Cu（II）配合物：水团簇的形成和大气二氧化碳的固定
3. Efficient and Mild Carbon Dioxide Hydrogenation to Formate Catalyzed by Fe(II) Hydrido Carbonyl Complexes Bearing 2,6-(Diaminopyridyl)diphosphine Pincer Ligands [J] . Bertini Federica, Gorgas Nikolaus, Stoeger Berthold, ACS catalysis . 2016,第5期

机译：含2,6-（二氨基吡啶基）二膦夹钳配体的Fe（II）氢羰基配合物催化高效轻度二氧化碳加氢形成甲酸酯
4. pH-Dependent Fixation of Carbon Dioxide by Water-Soluble Ruthenium Hydride Complexes [C] . Seiji Ogo, Hideki Hayashi, Tsutomu Abura, Symposium on Organometallic Chemistry . 2003

机译：水溶性钌络合物通过水溶性钌二氧化碳固定
5. New designs of rigid pincer ligands (PNP and PCP) and their transition metal complexes in the context of formation of M=C (M-carbene) moiety, strong bond activation (carbon-hydrogen, nitrogen-carbon, carbon-chloride) and catalysis [D] . Weng, Wei 2006

机译：刚性钳位配体（PNP和PCP）及其过渡金属络合物在M = C（M-卡宾）部分形成，强键活化（碳-氢，氮-碳，氯化碳）和催化作用下的新设计
6. Remarkable catalytic activity of dinitrogen-bridged dimolybdenum complexes bearing NHC-based PCP-pincer ligands toward nitrogen fixation [O] . Aya Eizawa, Kazuya Arashiba, Hiromasa Tanaka, -1

机译：带有基于NHC的PCP-钳位配体的氮桥联二钼配合物对固氮的显着催化活性
7. Divergent stereoisomers of molybdenum carbonyl complexes of NHC-based pincer ligands [O] . Apps, Samantha L., Alflatt, Rhiannon E., Leforestier, Baptiste, 2017

机译：基于NHC的钳型配体的羰基钼钼配合物的立体异构体
8. Carbon Monoxide and Carbon Dioxide Fixation: Relevant C1 and C2 Ligand Reactions Emphasizing (eta5-C5H5)Fe-Containing Complexes [R] . Cutler, A. R., Hanna, P. K., Vites, J. C. 1988

机译：一氧化碳和二氧化碳固定：相关的C1和C2配体反应强调（eta5-C5H5）含铁配合物

Fixation of atmospheric carbon dioxide by ruthenium complexes bearing an NHC-based pincer ligand: formation of a methylcarbonato complex and its methylation

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