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Probing the light hole/heavy hole switching with correlated magneto-optical spectroscopy and chemical analysis on a single quantum dot

机译:用相关磁光光谱探测灯孔/重孔切换和单量子点的化学分析

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A whole series of complementary studies have been performed on the same single nanowire containing a quantum dot: cathodoluminescence spectroscopy and imaging, micro-photoluminescence spectroscopy under magnetic field and as a function of temperature, and energy-dispersive x-ray spectrometry and imaging. The ZnTe nanowire was deposited on a Si3N4 membrane with Ti/Al patterns. The complete set of data shows that the CdTe quantum dot features the heavy-hole state as a ground state, although the compressive mismatch strain promotes a light-hole ground state as soon as the aspect ratio is larger than unity (elongated dot). A numerical calculation of the whole structure shows that the transition from the heavy-hole to the light-hole configuration is pushed toward values of the aspect ratio much larger than unity by the presence of a (Zn, Mg)Te shell, and that the effect is further enhanced by a small valence band offset between the semiconductors in the dot and around it.
机译:已经在含有量子点的相同单纳米线上进行了全系列互补性研究:在磁场下的阴极发光光谱和成像,微光致发光光谱和作为温度的函数,以及能量分散的X射线光谱和成像。 Znte纳米线用Ti / Al图案沉积在Si3N4膜上。 完整的数据集显示CDTE量子点具有作为接地状态的重孔状态,尽管一旦纵横比大于统一(细长点)就促进了光孔接地状态。 整个结构的数值计算表明,通过存在(Zn,mg)Te壳体的宽高比,从重孔与光孔构造的转变被推朝高于统一的纵横比的值。 通过点和周围的半导体之间的小价带偏移进一步增强了效果。

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