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Field effect transistors and phototransistors based upon p-type solution-processed PbS nanowires

机译:基于P型溶液处理的PBS纳米线的场效应晶体管和光电晶体管

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摘要

We demonstrate the fabrication of solution processed highly crystalline p-type PbS nanowires via the oriented attachment of nanoparticles. The analysis of single nanowire field effect transistor (FET) devices revealed a hole conduction behaviour with average mobilities greater than 30 cm(2) V (1) s (1), which is an order of magnitude higher than that reported to date for p-type PbS colloidal nanowires. We have investigated the response of the FETs to near-infrared light excitation and show herein that the nanowires exhibited gate-dependent photo-conductivities, enabling us to tune the device performances. The responsivity was found to be greater than 10(4) AW(-1) together with a detectivity of 1013 Jones, which benefits from a photogating effect occurring at negative gate voltages. These encouraging detection parameters are accompanied by relatively short switching times of 15 ms at positive gate voltages, resulting from a combination of the standard photoconduction and the high crystallinity of the nanowires. Collectively, these results indicate that solution-processed PbS nanowires are promising nanomaterials for infrared photodetectors as well as p-type nanowire FETs.
机译:我们证明的溶液的制造通过纳米颗粒的定向附接处理的高结晶性的p型的PbS纳米线。单个纳米线场效应晶体管的分析(FET)器件揭示了与平均迁移率超过30cm大的空穴传导行为(2)V(1)S(1),这是一个数量级比迄今报道的对于p更高型的PbS胶体纳米线。我们已经调查了FET的对近红外光激励的响应,并且在本文所述的纳米线表现出栅极依赖性光电导率,使我们能够调整器件性能显示。响应度被发现与1013琼斯的探测,其处出现负的栅极电压从photogating效果益处大于10(4)AW(-1)一起是。这些令人鼓舞的检测参数是伴随着在正栅极电压相对短的开关的15毫秒的时间中,从标准光电导和纳米线的高结晶度的组合产生的。总的来说,这些结果表明,溶液处理的纳米线的PbS,是约定的红外探测器,以及p型纳米线FET的纳米材料。

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