In situ growth of ZIF-67 on a nickel foam as a three-dimensional heterogeneous catalyst for peroxymonosulfate activation

Peng Lin; Gong Xiaobo; Wang Xinghong; Yang Zhao; Liu Yong

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In situ growth of ZIF-67 on a nickel foam as a three-dimensional heterogeneous catalyst for peroxymonosulfate activation

机译：原位生长ZIF-67在镍泡沫上作为过氧键硫酸盐活化的三维异质催化剂

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Advanced oxidation processes based on sulfate radicals have been widely used to eliminate contaminants. In this study, an efficient cobalt-based three-dimensional heterogeneous catalyst was fabricated through in situ growth of ZIF-67 on nickel foam (NF/ZIF-67). The factors influencing NF/ZIF-67-activated peroxymonosulfate (PMS) were investigated. Enhanced RhB degradation was observed using NF/ZIF-67-activated PMS under neutral conditions and high temperatures. Sulfate radicals were the dominant active species for the oxidative decolorization of RhB with NF/ZIF-67-activated PMS. NF/ZIF-67 was easily separated from the solution, and it also retained high catalytic stability. This study provides a rapid and mild method for the fabrication of promising three-dimensional heterogeneous catalysts for PMS activation and wastewater treatment.

机译：基于硫酸盐自由基的先进氧化方法已被广泛用于消除污染物。在该研究中，通过在镍泡沫（NF / ZIF-67）上原位生长来制造有效的基于钴的三维异质催化剂。研究了影响NF / ZIF-67活化的过氧键硫酸盐（PMS）的因素。使用NF / ZIF-67活化的PMS在中性条件下和高温下观察到增强的RHB降解。硫酸盐基团是用NF / ZIF-67活化的PMS氧化氧化脱光的主要活性物质。 NF / ZIF-67容易与溶液分离，并且还保留了高催化稳定性。该研究提供了一种快速和温和的方法，用于制造有希望的三维异质催化剂，用于PMS活化和废水处理。

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《RSC Advances》 |2018年第46期|共6页
作者
Peng Lin; Gong Xiaobo; Wang Xinghong; Yang Zhao; Liu Yong;
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Sichuan Normal Univ Coll Chem &

Mat Sci Chengdu 610066 Sichuan Peoples R China;

Sichuan Normal Univ Coll Chem &

Mat Sci Chengdu 610066 Sichuan Peoples R China;

Sichuan Normal Univ Coll Chem &

Mat Sci Chengdu 610066 Sichuan Peoples R China;

Sichuan Normal Univ Coll Chem &

Mat Sci Chengdu 610066 Sichuan Peoples R China;

Sichuan Normal Univ Coll Chem &

Mat Sci Chengdu 610066 Sichuan Peoples R China;

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正文语种 eng
中图分类化学;
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1. In situ growth of ZIF-67 on a nickel foam as a three-dimensional heterogeneous catalyst for peroxymonosulfate activation [J] . Peng Lin, Gong Xiaobo, Wang Xinghong, RSC Advances . 2018,第46期

机译：原位生长ZIF-67在镍泡沫上作为过氧键硫酸盐活化的三维异质催化剂
2. Application of nickel foam-supported Co_3O_4-Bi_2O_3 as a heterogeneous catalyst for BPA removal by peroxymonosulfate activation [J] . Hu Limin, Zhang Guangshan, Liu Meng, The Science of the Total Environment . 2019,第PTa1a1664期

机译：泡沫镍负载的Co_3O_4-Bi_2O_3作为非均相催化剂在过氧单硫酸盐活化去除BPA中的应用
3. Nanostructured CO_3O_4 grown on nickel foam: An efficient and readily recyclable 3D catalyst for heterogeneous peroxymonosulfate activation [J] . Yuan Ruixia, Hu Lin, Yu Peng, Chemosphere . 2018,第MAY期

机译：在镍泡沫上生长的纳米结构CO_3O_4：一种高效且易于回收的3D催化剂，用于非均相过氧单硫酸盐活化
4. Co~(2+)-Exchanged Titanate Nanotubes as a Novel Heterogeneous Catalyst for Peroxymonosulfate Activation and Degradation of Organic Pollutants [C] . Yun-Chen DU, Yan-Wu QI, Di GUO, Annual International Conference on Advanced Material Engineering . 2016

机译：CO〜（2 +） - 将钛酸盐纳米管交换为新型非均相催化剂，用于过氧键硫酸盐活化和有机污染物的降解
5. Activation of Hydrogen Peroxide by Iron-Containing Minerals and Catalysts in Circumneutral pH Solutions: Implications for ex situ and in situ Treatment of Contaminated Water and Soil. [D] . Pham, Anh Le Tuan. 2012

机译：周围环境pH溶液中含铁的矿物质和催化剂对过氧化氢的活化：对污水和土壤进行异位和原位处理的意义。
6. WS(1−x)Sex Nanoparticles Decorated Three-Dimensional Graphene on Nickel Foam: A Robust and Highly Efficient Electrocatalyst for the Hydrogen Evolution Reaction [O] . Sajjad Hussain, Kamran Akbar, Dhanasekaran Vikraman, 2018

机译：WS（1-x）Sex纳米颗粒在镍泡沫上修饰三维石墨烯：氢释放反应的鲁棒高效电催化剂
7. In situ autologous growth of self-supporting NiFe-based nanosheets on nickel foam as an efficient electrocatalyst for the oxygen evolution reaction [O] . Jianying Wang, Xue Teng, Yanli Niu, 2019

机译：在镍泡沫上的自支持NiFe纳米片的原位自体生长，作为氧气进化反应的有效电催化剂

In situ growth of ZIF-67 on a nickel foam as a three-dimensional heterogeneous catalyst for peroxymonosulfate activation

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