Heterogeneous Co-catalyzed direct 2-alkylation of azoles with ethers

Yang Ke; Li Dashan; Zhang Lei; Chen Qun; Tang Tiandi

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Heterogeneous Co-catalyzed direct 2-alkylation of azoles with ethers

机译：非均相辅助与醚的直接2-烷基化

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摘要

The direct 2-alkylation of oxazoles and thiazoles with ethers through cross-dehydrogenative coupling reaction using Co-containing mesoporous zeolite ETS-10 as the heterogeneous catalyst is described. The basic Co-containing mesoporous zeolite ETS-10 catalyst facilitates this cross-dehydrogenative coupling reaction through metal-base synergy catalytic principle.

机译：描述了通过使用共致孔沸石ETS-10作为非均相催化剂的含有共致脱氢偶联反应的醚与醚的二恶果和噻唑的直接2-烷基化。基本的Co-含型沸石ETS-10催化剂通过金属基础协同催化原理促进该交酯脱氢偶联反应。

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《RSC Advances》 |2018年第25期|共4页
作者
Yang Ke; Li Dashan; Zhang Lei; Chen Qun; Tang Tiandi;
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作者单位

Changzhou Univ Sch Petrochem Engn Jiangsu Key Lab Adv Catalyt Mat &

Technol 1 Gehu Rd Changzhou 213164 Jiangsu Peoples R China;

Changzhou Univ Sch Petrochem Engn Jiangsu Key Lab Adv Catalyt Mat &

Technol 1 Gehu Rd Changzhou 213164 Jiangsu Peoples R China;

Changzhou Univ Sch Petrochem Engn Jiangsu Key Lab Adv Catalyt Mat &

Technol 1 Gehu Rd Changzhou 213164 Jiangsu Peoples R China;

Changzhou Univ Sch Petrochem Engn Jiangsu Key Lab Adv Catalyt Mat &

Technol 1 Gehu Rd Changzhou 213164 Jiangsu Peoples R China;

Changzhou Univ Sch Petrochem Engn Jiangsu Key Lab Adv Catalyt Mat &

Technol 1 Gehu Rd Changzhou 213164 Jiangsu Peoples R China;

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正文语种 eng
中图分类化学;
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1. Heterogeneous Co-catalyzed direct 2-alkylation of azoles with ethers [J] . Yang Ke, Li Dashan, Zhang Lei, RSC Advances . 2018,第25期

机译：非均相辅助与醚的直接2-烷基化
2. Direct C2-alkylation of azoles with alcohols and ethers through dehydrogenative cross-coupling under metal-free conditions [J] . He T., Yu L., Zhang L., Organic letters . 2011,第19期

机译：在无金属条件下通过脱氢交叉偶联将唑类与醇和醚直接进行C2-烷基化
3. Silica sulfuric acid: An efficient catalyst for the direct conversion of primary and secondary trimethylsilyl ethers to their corresponding ethers under mild and heterogeneous conditions [J] . Zolfigol MA., Mohammadpoor-Baltork I., Mirjalili BF., Synlett . 2003,第12期

机译：二氧化硅硫酸：在温和和非均相条件下，伯和仲三甲基甲硅烷基醚直接转化为相应醚的有效催化剂
4. Synthesis and Preparation of Composite Membranes for Direct Methanol Fuel Cells from Poly(Ether Ketone Quinolines)-Poly(Ether Ether Ketone) Blend and Nafion with Non- and Surface Coated Silicotungstic Acid [C] . J. Sutrisno, I. Pramudya, A. Fuchs Direct alcohol fuel cells. . 2011

机译：聚（醚酮喹啉）-聚（醚醚酮）共混物和带有非表面和表面涂层硅钨酸的萘酚的合成和制备直接甲醇燃料电池用复合膜
5. Part I. Asymmetric organocatalysis: (1) Direct enantioselective organocatalytic hydroxymethylation of aldehydes catalyzed by alpha,alpha-diphenylprolinol trimethylsilyl ether: Application in the formal synthesis of (-)-Rasfonin; (2) Synthesis of a novel bicyclic secondary amine organocatalyst: Application to the direct enantioselective organocatalytic hydroxymethylation of aldehydes. Part II. Asymmetric synthesis of bicyclic analogues of the anti-osteoporotic drug risedronate. [D] . Miller, John Robert. 2010

机译：第一部分，不对称有机催化：（1）α，α-二苯基脯氨醇三甲基甲硅烷基醚催化的醛的直接对映选择性有机催化羟甲基化：在（-）-Rasfonin的正式合成中的应用；（2）新型双环仲胺有机催化剂的合成：应用于醛的直接对映选择性有机催化羟甲基化。第二部分抗骨质疏松药物Risedronate的双环类似物的不对称合成。
6. Inducible Azole Resistance Associated with a Heterogeneous Phenotype in Candida albicans [O] . Kieren A. Marr, Christopher N. Lyons, Kien Ha, 2001

机译：与白色念珠菌的异质表型相关的诱导性偶氮抗性。
7. Heterogeneous Co-catalyzed direct 2-alkylation of azoles with ethers [O] . Ke Yang, Dashan Li, Lei Zhang, 2018

机译：非均相辅助与醚的直接2-烷基化

Heterogeneous Co-catalyzed direct 2-alkylation of azoles with ethers

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